Bulletin of the Chemical Society of Japan
Online ISSN : 1348-0634
Print ISSN : 0009-2673
ISSN-L : 0009-2673
 
Experimental Studies and Redox-Type Monte Carlo Simulations for the Reduction Reaction of NO by CO over Supported Copper
Joaquín CortésEliana ValenciaCarlos GonzálezPaulo Araya
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2012 Volume 85 Issue 8 Pages 884-891

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Abstract

Kinetics experiments for the CO–NO reaction over copper oxide supported on zirconia are interpreted adequately by theoretical activity decay models. A redox-type reaction mechanism is proposed for the process. A kinetic Monte Carlo simulation algorithm is developed for the case of a redox mechanism. Its results give a reasonable interpretation of the order of the experimental reaction.

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© 2012 The Chemical Society of Japan
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