Bulletin of the Chemical Society of Japan
Online ISSN : 1348-0634
Print ISSN : 0009-2673
ISSN-L : 0009-2673
An Electron Spin Resonance Study of the Tropone Anion Radical
Yusaku IkegamiHidetoshi WatanabeShuichi Seto
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1972 Volume 45 Issue 7 Pages 1976-1978

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Abstract

The ESR spectrum of the tropone anion radical has been examined. The radical was generated from the neutral species by the electrolytic reduction in N,N-dimethylformamide. Splitting constants are satisfactorily explained in terms of the calculated spin densities by the McLachlan procedure, confirming that the unpaired spin orbital belongs to an a2 symmetrical species. The complete delocalization of the π-electrons was assumed for the anion radical.

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