Bulletin of the Chemical Society of Japan
Online ISSN : 1348-0634
Print ISSN : 0009-2673
ISSN-L : 0009-2673
Electronic Spectra and Electronic Structures of a Series of Bisdehydroannulenes
Jiro TanakaMasashi TanakaMasaharu MoritaMasazumi NakagawaMasahiko Iyoda
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1978 Volume 51 Issue 12 Pages 3458-3461

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Abstract

Electronic absorption spectra of tetra-t-butylbisdehydro[14], [18], [22], [26], and [30]annulenes were investigated experimentally and theoretically. SCF MO calculations were carried out by the P-P-P method and random phase approximation (RPA). An assignment of spectra is presented. Fluorescence excitation polarization spectra of tetra-t-butylbisdehydro[14]annulene and the crystalline reflection spectra of tetra-t-butylbisdehydro[18]annulene were studied in order to determine the polarization of the spectra. The assignment was confirmed by these methods.

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