Chemistry Letters
Online ISSN : 1348-0715
Print ISSN : 0366-7022
Letter
Solvent-mediated Tuning of the Regioselectivity of Intramolecular Diaryl Ether Formation: Total Synthesis of (+)-Aspercyclide C
Tatsuya YoshinoShuji YamashitaItaru SatoYujiro HayashiMasahiro Hirama
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Volume 43 (2014) Issue 3 Pages 349-351

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Abstract

A concise total synthesis of the 11-membered cyclic (+)-aspercyclide C is reported. Key to success was the fine-tuning of the reaction media to realize an oxidative, macrocyclic diaryl C–O bond formation in a regioselective and direct fashion.

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© 2014 The Chemical Society of Japan
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