Chemistry Letters
Online ISSN : 1348-0715
Print ISSN : 0366-7022
ISSN-L : 0366-7022
New Radical Anion Complex, [(CH3)4N][Ni(dmit)2]2 with Metal-Semimetal Phase Transition
Hyernjoo KimAkiko KobayashiYukiyoshi SasakiReizo KatoHayao Kobayashi
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1987 Volume 16 Issue 9 Pages 1799-1802

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Abstract

The crystal structure determination was made on the multi-sulfur π-acceptor complex, [(CH3)4N][Ni(dmit)2]2, which is the first molecular metal composed of Ni(dmit)2 (dmit=isotrithionedithiolate) molecules and the closed-shell cations. The metal-semimetal transition with large hysteresis was observed.

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