有機合成化学協会誌
Online ISSN : 1883-6526
Print ISSN : 0037-9980
ISSN-L : 0037-9980
総説および総合論文
可視光エネルギーを分子変換へ利用する金属錯体の開発
稲垣 昭子
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ジャーナル 認証あり

2022 年 80 巻 5 号 p. 489-497

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Utilization of light energy, especially visible-light energy, which can be gained inevitably from sunlight, has now attracted emerging attention due to the recent serious environmental issues. In the field of homogeneous catalysis, various efficient photoredox reactions have been developed, in which mainly ruthenium and iridium visible-light sensitizers play the key roles in the catalysis to promote single electron transfer to generate reactive radical species under mild conditions. Apart from these reactions, utilization of the excited-state of the catalyst itself may lead to the new type light-controlled reactions. In order to realize such reactions, precise design of the photocatalysts is inevitable for the efficient formation of the desired excited-state. Here, we will introduce our intensive studies on developing the visible-light driven catalysts.

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