Two markedly different trends of evolution of biotites were found in the granitic rocks of Southwest Japan.
(1) Late Mesozoic to early Tertiary granites: The iron/magnesium ratios in both rocks and biotites increase with decreasing solidification index (SI). The difference of the ratio between rocks and biotites is small. The magnetite content in the granities is below 1.5 per cent usually.
(2) Palaeogene Tamagawa plutonic rocks: As the differentiation progresses, the iron/magnesium ratio has a similar trend as that in (1) from gabbro to granodiorite in both biotites and rocks, whereas from granodiorite to granite the ratio becomes reversed in the biotites due to their turning into magnesium rich compositions. The content of magnetites is high, amounting to 4 per centor more. They replace biotites and form interstitial fillings.
On the basis of physico-chemical aspects, it is assigned that the oxygen partial pressure during the evolution of biotites has been under slightly decreasing c on dition in the late Mesozoic to early Tertiary granites, while almost constant or somewhat in creased in the Tamagawa plutonic rocks in which at leasta part of the oxygen are presumed to have been derived from atmosphere, although its invading process is quitely questionable. The latter case is common in the plutonics of the cauldron subsidence area.
The reaction series of the constituent minerals for the Tamagawa plutonic rocks is conspicuously differed from ordinary types of granite belonging to calc-alkaline rock series as shown in Fig. 17.
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