In this paper, we report experimental results on the overall magnetic properties of intermetallic compounds Gd
1-xLa
xMn
2Ge
2 (0≤
x≤1.0) with a ThCr
2Si
2-type layered structure. In GdMn
2Ge
2, a first order transition was observed from antiferromagnetic to ferrimagnetic state at
Tt3 below
TN with decreasing temperature, while in Gd
1-xLa
xMn
2Ge
2 with
x = 0.075 and 0.050, two kinds of first-order transitions, from ferrimagnetic to antiferromagnetic and from antiferromagnetic to reentrant ferrimagnetic states were observed at
Tt2 and
Tt3 after they become ferrimagnetic below
Tt1. As
x further increases canted ferrimagnetism appears with a compensation temperature in all the ordering temperature regions for 0.10 <
x < 0.40, whereas no compensation behavior was observed for
x > 0.50. The compensation behavior as a function of temperature is discussed on the basis of the two-sublattice molecular-field model.
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