Cold spray (CS) technique is a method of particle deposition. Particles, which are accelerated by a high-speed gas flow and collide with the substrate at supersonic speed, are plastically deformed and deposited to the substrate. Cold spray technique has been developed to fabricate polyethylene (PE) and carbon nanotube (CNT) composite film. In this research, the relative angle between nozzle and substrate (θ) was varied to align the CNTs in the composite films. PE-CNT composite films were fabricated on polypropylene substrate at θ = 0,5 and 10°. CNTs were moderately aligned vertically at θ = 0°. At θ = 5 and 10°, the CNTs were oriented around 55°. Electrical conductivity was improved at θ = 10°.