JJAP Conference Proceedings
Online ISSN : 2758-2450
2nd Japan-China Joint Workshop on Positron Science (JWPS2013)
Session ID : 011003
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Theory and related experiments on physics and chemistry
Positronium bubble oscillation in room temperature ionic liquids
Tetsuya Hirade
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CONFERENCE PROCEEDINGS OPEN ACCESS

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Abstract

Positronium bubble oscillation before the stabilization of the bubble was successfully observed by the change of the triplet Ps (ortho-Ps) pick-off annihilation rate in a room temperature ionic liquid, N,N,N-trimethyl-N-propylammonium bis(trifluoromethanesulfonyl)imide (TMPA-TFSI). It was reported that the Ps bubble stabilization in TMPA-TFSI took more than 500 ps. For materials having Ps formation, singlet Ps (para-Ps) gives the fastest annihilation mean lifetime of about 125 ps. Although it is intrinsic annihilation, the Ps bubble oscillation affects the para-Ps annihilation rate. The oscillation on the ortho-Ps pick-off annihilation was expected to appear at positron ages older than about 400 ps after the para-Ps annihilation fraction becomes small enough. An oscillation with 5.85 GHz frequency of the ortho-Ps pick-off annihilation rate was successfully observed at the positron ages older than 500 ps in 25 °C TMPA-TFSI.

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