Abstract
he 51V NMR in L21-type Fe2Vsi was measured as a function of temperature using the spin-echo method. The 51V Knight shift was 0.115% at 10~K. The 51V NMR spectra in applied fields have unusually broadened tails. This suggests the existence of Fe atoms with relatively large magnetic moments due to atomic disorders. The atomic disorders between Fe sites and other atomic sites were indicated by the observation of the broad X-ray diffraction lines corresponding to (100) and (110).