2000 Volume 69 Issue 11 Pages 3521-3524
The direct electron spin resonance (ESR) absorption between a singlet ground state and the triplet excited states of spin gap systems is investigated. Such an absorption, which is forbidden by the conservation of the total spin quantum number in isotropic Hamiltonians, is allowed by the Dzyaloshinskii-Moriya interaction. We show a selection rule in the presence of this interaction, using the exact numerical diagonalization of the finite cluster of the quasi-one-dimensional bond-alternating spin system. The selection rule is also modified into a suitable form in order to interpret recent experimental results on CuGeO3 and NaV2O5.
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