Journal of the Physical Society of Japan
Online ISSN : 1347-4073
Print ISSN : 0031-9015
ISSN-L : 0031-9015
Filling Control of the Mott Insulator Ca2RuO4
Hideto FukazawaYoshiteru Maeno
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2001 Volume 70 Issue 2 Pages 460-467

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Abstract
We have grown single crystals of electron doping system Ca2-xLaxRuO4 (0.00 ≤ x ≤ 0.20) by a floating zone method. The first order metal/non-metal transition and canted antiferromagnetic ordering occur for 0.00 < x < 0.15, similar to those in the bandwidth controlled system Ca2-xSrxRuO4 (CSRO). However, comparing with CSRO, we found a rather different metallic ground state adjacent to the non-metallic ground state with canted antiferromagnetic order. Instead of short-range antiferromagnetic correlation found in CSRO (0.20 ≤ x < 0.50), the metallic ground state of the present system is characterized by strong ferromagnetic correlation.
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© The Physical Society of Japan 2001
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