Three new furanoeremophilanes were isolated from Ligularia japonica Less., and their structures determined as furanoeremophilane-6β, 10β-diol (I), 10β-hydroxy-6β-methoxyfuranoeremophilane (II) and 10β-hydroxyfuranoeremophilan-6β-y1 2'ζ-methylbutanoate (III), respectively. Two new sesquiterpenes isolated from Farfugium japonicum Kitam. (=Ligularia tussilaginea Makino) were shown to be a tetrahydronaphtofuran derivative (V) and a benzofuran derivative (VI), respectively.