2022 年 36 巻 4 号 p. 423-431
The objective of this study is to elucidate the formation and growth behavior of CO2 hydrate. Based on hydrate film thickness measurements, the process of hydrate film development was classified into "formation" and "growth". A macro-scale thickness prediction model based on mass transport was constructed for these processes. Molecular dynamics calculations were also introduced and combined with the macro-scale prediction model to construct a model capable of predicting film thickness.