Journal of the Physical Society of Japan
Online ISSN : 1347-4073
Print ISSN : 0031-9015
ISSN-L : 0031-9015
Spin-Gap Behavior of CuNb2O6
Katsuaki KodamaToshihiko FukamachiHiroshi HarashinaMasaki KanadaYoshiaki KobayashiMayumi KasaiHisashi SasakiMasatoshi SatoKazuhisa Kakurai
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1998 年 67 巻 1 号 p. 57-60

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The magnetic properties of two polymorphs of CuNb2O6 with quasi-one-dimensional zig-zag spin (S=1/2) chains of Cu2+ ions are studied. The magnetic excitation spectra of Cu spins measured by neutron scattering, and the T-dependence of the longitudinal spin relaxation rate of 93Nb nuclei by NMR indicate the existence of the spin gap in the monoclinic phase whose magnitude is consistent with the one deduced by the detailed analyses of uniform magnetic susceptibility at low temperatures. The behavior in the monoclinic phase is in clear contrast to that found in the orthorhombic phase.

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© The Physical Society of Japan 1998
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