Journal of the Physical Society of Japan
Online ISSN : 1347-4073
Print ISSN : 0031-9015
ISSN-L : 0031-9015
Two Spin Ordered States under a Magnetic Field along Different Crystalline Axis in Ni(NO3)2·4H2O
Nobuo WadaKoh MatsumotoKiichi AmayaTaiichiro Haseda
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1978 年 45 巻 5 号 p. 1771-1772

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The crystal of Ni (NO3)2·4H2O is found to contain two kinds of sites for Ni2+ ions in a unit cell. By the measurements of the isentrope, susceptibility and specific heat, two spin ordered states are observed applying a field along either of the two ion axes, zA and zB, corresponding to the two inequivalent Ni2+ sites. One of the spin orderings occurs between 12 kOe and 44 kOe (H⁄⁄zA) and the other at a higher field region than 35 kOe (H⁄⁄zB). The highest critical temperature is 0.57 K (H⁄⁄zA), and is lower than this when H⁄⁄zB.
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