Abstract
NMR signals of 27Al in the commensurable state of CrAl alloys were observed at liquid He temperatures. The hyperfine field at Al site due to the magnetic moment of Cr atom is about 32 kOe/μB. The hyperfine field of 27Al increases with increasing Al concentration almost in proportion to the average magnetic moment. The nuclear spin-lattice relaxation time, T1, has been also measured under the same condition. The product of T1 and the temperature, T1T, increases with Al content.