レーザー研究
Online ISSN : 1349-6603
Print ISSN : 0387-0200
ISSN-L : 0387-0200
レーザー解説
固体高次高調波発生の理論と第一原理計算
石川 顕一篠原 康
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ジャーナル フリー

2020 年 48 巻 4 号 p. 162-

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抄録
Solid-state materials have recently emerged as a new stage of strong-field physics and attosecond science. The mechanism of high-harmonic generation (HHG) from solids is being scrutinized. Here we theoretically discuss the momentum-space pictures of HHG from graphene and crystalline dielectrics and semiconductors. Within massless Dirac fermion and tight-binding models, we rigorously derive intraband displacement and interband transition, which form the basis for understanding solid-state HHG. Then based on the results of simulations that solve the time-dependent Schrödinger equation for a one-dimensional model crystal, we introduce a simple momentum-space three-step model that incorporates intraband displacement, interband tunneling, and recombination with a valence band hole. We also present a time-dependent density-matrix method that simulates HHG from actual three-dimensional materials whose results are compared with experiments to increase the understanding of measurement results.
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© 2020 一般社団法人 レーザー学会
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