The vertical distributions of the
14C
137CS
210Pb, and
214Pb concentrations, and of total organic carbon and nitrogen contents, were examined for the 50cm-long cored sediment collected from Lake Biwa(35. 3°N, 136°E, water depth: 70m). The sediment column was divided by 5mm intervals from surface to 10cm depth and by 10mm from 10 to 30cm depth. The
14C abundance, Δ
14C, was measured by the direct detection of
14C atoms using a Tandetron accelerator mass spectrometer on acid-insoluble organic carbon extracted from 1.5g of each sediment sample divided vertically. Activities of
137Cs,
210Pb and
214Pb were measured with a well-type pure-germanium detector, and the total organic carbon and nitrogen contents with a C-N corder, using about lg of each sample.
The followings were revealed through the present study:
(1) The sedimentation rate was calculated to be 0.0333±0.002g/cm
2/yr(0.152±0.008cm/yr at the surface of the bottom sediment) by the
210Pb method. The flux of 210Pb
excessdeposition at the surface of the bottom sediment was 0.45±0.04pCi/cm
2/yr; this was about 60% of the annual
210Pb deposition from the atmosphere.
(2) The
137Cs concentration was widely distributed through the sediment column in comparison with a yearly change of the deposition rate from the atmosphere. The total amount of
137Cs deposited in the sediment column was calculated as 2.63pCi/cm
2; this was about 65% of the amount of total
137Cs deposited so far in Osaka.
(3) Both organic carbon and nitrogen contents of the sediment decreased rapidly with increasing depths and reached constant values around 8-9cm in the depth. On the other hand, the carbon to nitrogen ratio was almost constant (C/N≈10) throughout the sediment column studied.
(4) The Δ
14C value of the sediment increased from-250 to 40‰, with changing depths from 3cm to surface, owing to the addition of the artificially produced
14C to the atmosphere. The Δ
14C value of the sediment before nuclear tests was about-250‰; this
14C concentration was 25% lower than that of the atmospheric CO
2 at that time. The increase in the
14C concentration of the sediment due to the bomb produced
14C was monotonous, lasting from 1956 to 1980. This change of Δ
14C with time showed a quite different trend from the yearly change of Δ
14C of the atmospheric CO
2, depending probably on the complicated mechanism of accumulating organic materials in the lake sediments.
(5) Radiocarbon dating on organic carbon of Lake Biwa sediments at depths from 3 to 4cm gave the
14C ages of 2200-2400y BP, which were quite older than the
210Pb ages of A. D. 1945-55.
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