Bamboo–plastic direct bonding was attempted via a fused deposition modelling (FDM) typed three-dimensional (3D) printer, aiming to enhance bamboo use. Polylactic acid (PLA) filaments were employed in 3D printing, and bamboo specimens were grooved via laser processing, hoping to attain the anchoring effect that provides a strong physical bonding. Because such many process parameters that are practically impossible to verify all the combinations of them exist, three parameters, the laser power (P), hatch spacing (h), and temperature of the 3D printer nozzle (θ), were selected and a Taguchi L9 orthogonal array was used to reduce the number of trials. The experimental results illustrated that P is the main effect for the depth of the laser grooves and h and interaction P×h are weaker but still significant effect. All the laser-grooved specimens demonstrated larger tensile strengths than the control specimens on average. From the main effect plot of the Taguchi method, the optimal conditions were P = 60% (of nominal maximum output, 20 W), h = 1.0 mm, and θ = 210°C within the experimental range. At the low laser power, P = 40%, insufficient penetration of PLA into the grooves led to lowering the tensile strength due to delamination at the bonding interface. Conversely, At the high laser power, P = 80%, and the narrow hatch spacing, h = 0.5 mm, the heat affected significantly onto the bamboo specimens and the islands of the hatch pattern were easily destroyed, resulting in decrease in the tensile strength.
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