Materials and Systems Design for Energy Conversion with CO₂ Separation and Utilization Using Chemical-looping Technology

Abstract

To achieve net-zero CO₂ emissions over the coming decades, innovative new technologies, including separation, storage, and utilization of CO₂, are indispensable. Chemical looping technology may provide effective solutions and promising energy conversion systems for power plants and industrial applications with inherent CO₂ capture, avoiding energy penalties. Combined with appropriate CO₂ storage and utilization options, chemical looping can achieve net-zero emissions. The challenges, benefits, and prospects of chemical looping systems with various oxygen carriers and reactor configurations are discussed in this review to provide insights into the development of innovative systems in terms of solid looping materials, reactions, systems, and economics.