1972 年 33 巻 1 号 p. 39-48
Temperature dependent absorption strength of several absorption bands of MnF2 and RbMnF3 in visible and ultra-violet region is investigated experimentally and theoretically. The oscillator strength for the exciton-magnon transitions increases as temperature increases up to Néel temperature TN or even above TN, and saturates or varies only slightly at higher temperatures. It is found, however, that the temperature dependence of the cold band intensity below TN is quite different from this as expected from the theory. The temperature variation of the intensity of the two-exciton transitions is somewhat similar of that of the cold band, namely, the intensity starts to decrease with the increase of T below TN and is nearly constant or increases slightly above TN.
Theoretical explanations for these experimental results are presented. The calculation which assumes inter- and intrasublattice pair excitation leads to the results in qualitative agreement with the experiment. Causes of quantitative discrepancy are also discussed.
この記事は最新の被引用情報を取得できません。