Journal of the Physical Society of Japan
Online ISSN : 1347-4073
Print ISSN : 0031-9015
ISSN-L : 0031-9015
Spin Glass State of MnxNi1−xSb: Synthesis in High Pressure and High Temperature Atmospheres
Kengo AdachiRyo ImuraMasaaki MatsuiHiroshi Sawamoto
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1978 年 44 巻 1 号 p. 114-121

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The solid solution between ferromagnetic MnSb and paramagnetic NiSb, MnxNi1−xSb (0≤x≤1.0), with NiAs structure was synthesized in high pressure and high temperature atmospheres. The decomposition temperature was determined to be 420∼480 K. The critical concentration of ferromagnetism was obtained to be xc=0.65 at absolute zero. A new type spin glass state with double transition points, Tsg1 and Tsg2, was found in a wide range of 0.2≤x≤0.65 in the paramagnetic phase. The maximum transition point was estimated to be Tsg1=60 K and Tsg2=190 K. The electrical resistivity showed no anomaly corresponding to Tsg1 and Tsg2, and the temperature dependence in the spin glass state was given to be T2 and T3⁄2 at lower temperature. Some discussions are given for the experimental results.
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