1990 年 59 巻 6 号 p. 1932-1935
We observed the temperature and the x-dependence of the 139La-NQR spectra in magnetically ordered La2−xBaxCuO4. The internal field at La nuclei increases discontinuously at Tc*, where the nuclear relaxation rate is enhanced and shows its peak. This indicates that a successive magnetic transition occurs at Tc* for x<0.02. An asymmetry parameter of the electric quadrupole interaction changes anomalously at the magnetic transition. The magnetic phase diagram of the La-system is discussed.
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