e-Journal of Surface Science and Nanotechnology
Online ISSN : 1348-0391
ISSN-L : 1348-0391

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Layer-selective Optical Second-harmonic Generation Spectroscopy of a MoS2/WSe2 Heterobilayer
Yoshihiro Miyauchi Yasuyuki HirataShinya Ohno
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ジャーナル オープンアクセス 早期公開

論文ID: 2025-013

この記事には本公開記事があります。
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The so-called C exciton resonance enhancement peak for heterostructures (HSs) of transition-metal dichalcogenides is indicative of a change in the band structure due to interlayer coupling. However, the superposition of the broad C exciton peaks from the two layers presents a significant challenge to the analysis of the alteration. The aim of this study was to gain insight into the electronic states of the C exciton region in each layer of a MoS2/WSe2 HS. To this end, we obtained second-harmonic generation (SHG) spectra of the HS by fixing the incident polarization angle to sequentially minimize the second-harmonic signals from the WSe2 and MoS2 layers. The resulting SHG spectra comprised signals from the MoS2 (former case) and WSe2 layers (latter case), demonstrating that the C exciton peak from each layer of the HS could be observed individually.

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