We have analyzed in detail an episode of PM
2.5 from 4 to 7 February 2011 over Japan. The peak time of the PM
2.5 concentration was delayed from west to east along the Sea of Japan on February 4th. High concentrations of PM
10 were observed in Korea on February 3rd. A backward trajectory analysis and satellite data showed that the air mass from Mainland China arrived at many sites in Japan. PM
2.5 filter samples were collected at ten sites during the high concentration episode. The chemical composition of PM
2.5 at Miyazaki and Okayama did not change during the episode. On the other hand, the ratio of sulfate, nitrate and ammonium to PM
2.5 had increased in direct proportion to the PM
2.5 concentration during the episode on the east side. The ratio of NO
3-/SO
42- was the lowest for the trans-boundary air pollution. The ratio of NO
3-/SO
42- was higher at the urban site for urban pollution. Based on these results, it was suggested that the high concentrations of PM
2.5 were caused by trans-boundary pollution as well as domestic pollutants in the urban areas.
View full abstract