Equilibrium particle size distributions of the stratospheric aerosol are investigated assuming two production mechanisms. When many stratospheric aerosol particles are produced in the local homogeneous nucleation and are removed by diffusion from the stratosphere (model 1), their size distribution is characterized by three spectral ranges A (
r_??_0.01μm), B (0.01μm _??_
r_??_0.1μm), and C (
r_??_0.1μm). The particles in the range A are controlled mainly by coagulation and the spectrum is proportional to
r-2.75. The particles in the range C grow in size by the attachment with smaller particles and are removed from the stratosphere by sedimentation and eddy diffusion. Coagulation between large particles is negligible because their concentration is small (-1cm
-3). The spectrum in the range C is calculated based on the condensational growth model and is compared with the results of measurements using impactors. The calculation of the spectrum in the range B is not easy because all physical processes are involved, and the spectrum is strongly dependent on the nucleation rate as well as interaction with particles in the range C. This model will be valid when H
2SO
4-HNO
3-H
2O ternary particle formation effectively takes place or where H
2SO
4-H
2O binary formation is activated due to the intrusion of dense water vapor from the upper troposphere near the jet stream or by another air exchange between the troposphere and the stratosphere.
In model 2, Aitken particles transported into the stratosphere from the troposphere or from meteoric flux grow in size by heteromolecular condensation of H
2SO
4-H
2O vapor, and are removed by diffusion from the stratosphere into the troposphere. In this model, which will be valid for the average state of the lower stratosphere even when HNO
3 molecules do not take part in the formation, new particles are not produced in the stratosphere. Concentrations of Aitken particles originated from the troposphere decrease going upwards, and the mean radius of the particles becomes greater. These features are consistent with the measurements of Wyoming group. However the size spectrum of Aitken particles determined by PODZIMEK
et al. (1977) does not support model 2 and its shape is similar to model 1. To establish the size spectrum is urgently needed.
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