A basic study was performed on the mass spectrometric determination of burnup for a UO
2 specimen irradiated in the HFR. It has been found that:
(1) By isotopic analysis of uranium, the contribution to burnup provided by the specimen through fissioning of
235U was determined to be 4, 370 MWD/T. The loss of
235U through neutron capture was distinguished by the production of
236U.
(2) The contribution to burnup of the specimen by fissioning of
239Pu was determined to be 3, 610 MWD/T from the excess formation of fission products such as
93Zr, based on the known number of
235U fissions.
(3) The total burnup of the UO
2 specimen was taken to be 7, 980 MWD/T, since no other isotopes of plutonium were identified.
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