In an aerated soil layer under natural condition, water that infiltrates into it flows discontinuously because of repeated cycles of rainfall and drying. Therefore, column tests, in which 2, 000 ml of deionized water was fed into sandy soil layer dried for 390 days after it is conaminated by
60Co,
85Sr and
137Cs aqueous solution, were carried out to examine influence of the drying period on migration behavior of those nuclides.
All the radionuclides showed both a steeply decreasing part corresponding to their cationic form and a gradually decreasing part corresponding to their particulate form in the concentration distribution curve along the soil column depth. In the vicinity of the top surface of soil layer, no influence of drying on
60Co and
137Cs concentrations was observed, but
86Sr moved a little into a deeper part from the top surface with longer drying period. Such moving tendency of
85Sr was found to be connected with the Ca
2+ concentration in the interstitial water. In the deeper soil layer, no influence of drying on
85Sr concentration was observed, but the
60Co and
137Cs concentrations were increased with the drying period. This is considered to be caused from that each product of the movable
60Co(OH)
2 and the
137Cs adsorbed on the fine particle increased with the rise of pH and the fine particle concentration, respectively, during the drying period. Thus, this study has suggested possible causes affecting on the radionuclide migration under discontinuous flow condition.
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