"Dorozome" is one of the traditional dying methods with muddy clays in Amami-Ohshima Island, Kagoshima, Japan. The brilliant black color of dyed "Ohshima Tsumugi" derives from muddy clays in Dorota (small ponds with muddy clays). In this paper, muddy clays for dying were mineralogically, chemically and microbiologically characterized. The muddy clays consist of Fe-rich chlorite, vermiculite, mica clay minerals, kaolin minerals as well as a large amount of iron hydroxides associated with high P2O5, N, C and S contents in the muddy field. Principally, iron is a key element which constitutes not only crystalline/amorphous hydroxides iron minerals, but also clay minerals. After one year of using the muddy clays, the Eh and DO are significantly reduced in fallow field. Various microorganisms were observed in the muddy clays, such as coccus and bacillus typed bacteria and fungi. Anaerobic bacteria may contribute for reducing condition in the muddy field. The black parts of "Ohshima Tsumugi" contain high concentrations of S, Ca and Fe, whereas white parts without dye contain a small amount of such elements. The heavy metals are originated from both muddy clays and Rhaphiolepis umbellata. The results suggest that specific condition of iron hydroxides is an important factor for brilliant black dye under reducing condition.
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