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Junsei Chiba, Ryugo S. Hayano, Michiko Sekimoto, Hisayoshi Nakayama, K ...
1977Volume 43Issue 4 Pages
1109-1118
Published: October 15, 1977
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Band structures of the
135La,
133La and
129Cs nuclei have been studied by means of in-beam γ-ray spectroscopy following the (α, 2n) and (
3He, 3n) reactions. The 11/2
− decoupled bands and positive-parity bands built on the 5⁄2
+ and 7/2
+ states have been observed. A new isomeric state of
129Cs with a half-life of 0.69±0.03 μsec has been discovered.
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Yuichi Iritani, Jirohta Kasagi, Hajime Ohnuma
1977Volume 43Issue 4 Pages
1119-1124
Published: October 15, 1977
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Low-lying excited states of
52Fe were investigated by using the
50Cr (
3He, nγ)
52Fe reaction at
E3He=8 MeV. A gamma-ray decay scheme has been proposed based on n-γ and γ-γ coincidence measurements. The lifetimes of four excited states, as well as the lower limit for the lifetime of the first excited state, have been obtained from the analysis of Doppler-shift attenuation measurements.
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Masakazu Ichiyanagi
1977Volume 43Issue 4 Pages
1125-1130
Published: October 15, 1977
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In the light of the Higgs mechanism in the spontaneous breakdown of symmetry, we discuss the properties of quantized vortex in superfluid helium. We introduce quantum mechanically the depletion velocity field which couples with particle fields. The coulping constant needs not be assumed to be equal to m, the mass of the (helium) particles. We will define the vorticity in terms of the depletion velocity instead of defining it by the gradient of the phase of the condensate wavefunction. A possibility of the half-integer quantum of vortices is suggested.
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Takashi Karasudani, Hisao Okamoto
1977Volume 43Issue 4 Pages
1131-1136
Published: October 15, 1977
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The temperature dependence of EPR frequencies is studied theoretically for pure and pseudo-one dimensional Heisenberg magnets by means of Mori’s theory of generalized Brownian motions. In a system with uniaxial symmetry, simple expressions for resonance frequencies are obtained. It is seen that the resonance frequencies are shifted from the Zeeman frequency when the magnetic susceptibility is anisotropic. Fisher’s classical spin model is used to calculate the spin correlation functions. The anisotropy of the magnetic susceptibility is found to be enhanced by an effect of the short range order. The pseudo-one dimensional systems are treated with the help of the mean field approximation to interchain interactions. The result is reduced to that of a pure-one dimensional system, when the interchain interactions are absent. The effects of interchain interactions are negligible for antiferromagnets even near the Néel point, whereas those for ferromagnets are divergent near the Curie point. Nagata and Tazuke’s expressions for a
g-shift can be obtained from the present theory in an approximation .
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Toshio Hyodo, Osamu Sueoka
1977Volume 43Issue 4 Pages
1137-1143
Published: October 15, 1977
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High momentum components in the momentum distribution of annihilation photons from Cu single crystal have been investigated using the crossed-slit rotating-specimen method. The obtained data have been analyzed by using a simple model based on the Wigner-Seitz approximation. Agreement of the calculated results with the experimental data is good in high momentum region, suggesting that, away from the zone boundaries, the “umklapp” annihilation rate does not strongly depend on the momentum. However, the observed intensity of the “umklapp” annihilation relative to the “normal” annihilation has been considerably smaller than that predicted by the Wigner-Seitz model.
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Hiroyuki Kaga
1977Volume 43Issue 4 Pages
1144-1153
Published: October 15, 1977
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X-ray edge singularities in the spin-dependent final-state interactions have been calculated perturbationally in the most divergent term approximation for the photoelectron and absorption spectra of the narrow-band metals (and also the simple metals). For the ferromagnetic exchange couplings (
J>0) of conduction electrons with the core-hole or the narrow-band electron spins
S, the exchange interaction is found to make the two different contributions: (i) the Mahan threshold singularity is modified by a logarithmic factor (1–2ρ
Jlog|ω⁄
D|)
η, and (ii) the Anderson orthogonality exponent is increased by ζ(ρ
J)
2, where η and ζ depend on the spin
S multiplicity, and ρ and
D are the density of states and the cut-off width of the conduction band, respectively. A possibility is pointed out that the edge singularities may be
suppressed at the absorption threshold of the transition metals.
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Kazuo Nakazato
1977Volume 43Issue 4 Pages
1154-1162
Published: October 15, 1977
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The boundary conditions of hydrodynamic equations are formulated by introducing a phase shift into each hydrodynamic mode of a linearized Boltzmann equation. Its rigorous treatments are shown, and an analytic form of the phase shift is obtained for the BGK model.
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Masaaki Kaminaga
1977Volume 43Issue 4 Pages
1163-1168
Published: October 15, 1977
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Approximate solutions of the nonlinear equation that describes the behavior of microwave-irradiated superconducting weak links are obtained. The method of the solution is based on the fact that the phase of Josephson oscillation is locked to an externally applied coherent radiation under a bias current of a microwave-induced step. It can be concluded that the approximate solutions have three internal variables which are functions of d.c. bias current and microwave current. The d.c. voltage-current relation when d.c. current is biased to a current step is found to follow Ohm’s law when the step vanishes. This result has been confirmed experimentally. The height of a current step as a function of the incident microwave current has been numerically calculated. The calculated values agree well with those obtained by an analog computer. The internal three variables have been also calculated numerically.
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Kazuyuki Matsui, Yoshika Masuda
1977Volume 43Issue 4 Pages
1169-1177
Published: October 15, 1977
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The host
27Al nuclear spin-lattice relaxation in the normal and superconducting states of the (La
1−nGd
n)
3 Al and (La
1−nCe
n)
3 Al systems has been studied for low impurity concentration and over wide ranges of temperature (1.2∼20 K) and field (6.8∼13.5 kOe). The measured relaxation rate 1⁄
T1 shows strong impurity concentration and field dependences in both the normal and superconducting states. An analysis of the experimental results indicates that the direct process induced by the longitudinal dipolar fluctuations of the localized magnetic impurity moment plays an important role. The results are compared with the pair breaking theory qualitatively in the vicinity of the superconducting transition temperature.
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Takeshi Kanomata, Takao Goto, Hideaki Ido
1977Volume 43Issue 4 Pages
1178-1184
Published: October 15, 1977
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Magnetic and crystallographic measurements on Fe
2.1−xMn
xAs with 0≤
x≤2.1 are made in the temperature range between 77 and 600 K. The compounds with 0≤
x<1.29 and 1.52<
x≤2.1 have the antiferromagnetic spin structures of the Fe
2As and Mn
2As types, respectively. The compounds with 1.29≤
x≤1.52 show a first order phase transition between the ferrimagnetic state of the Mn
2Sb type and the antiferromagnetic state of the Fe
2As type. A magnetic phase diagram of Fe
2−xMn
xAs system is proposed and discussed qualitatively on the basis of the molecular field theory.
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Tetsu Hiraki, Kazuo Ôno
1977Volume 43Issue 4 Pages
1185-1193
Published: October 15, 1977
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The nuclear orientation experiment on
54Mn nuclei in Au metal and Au(Cr), Au(Mn), and Au(Fe) alloys have been made to study the nature of the spin glass and the Kondo effect in these alloys. Concentrations of impurities in the alloys were between 5 and 500 at. ppm and measurements were performed in the temperature range between 7 and 8 mK. Gamma-ray anisotropy from oriented
54Mn in the Au(Mn) and Au(Cr) alloys can be explained by the 3-dimensional Lorentzian distribution function, when the molecular field approximation is applied to the spin glass state. For the Au(Fe) alloys, however, widths of the distribution function are less than those expected from the molecular field approximation, which may be attributed to the Kondo effect. Nuclear orientation of
54Mn in Au metal is explained by the slow relaxation model with S
Mn=5⁄2. This indicates that the Kondo temperature of Au(Mn) is lower than 7 mK.
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Fumihisa Ono
1977Volume 43Issue 4 Pages
1194-1199
Published: October 15, 1977
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A model for the temperature and the magnetization dependences of the magneto-crystalline anisotropy energy for Ni has been proposed based on the itinerant electron model by considering the effect of thermally excited magnons on the spin-orbit interaction. The temperature variation of
K1 at low temperatures can be expressed by the terms proportional to
T3⁄2,
T2 and
T5⁄2. Experimentally determined values of the coefficient of the term
T3⁄2 is 586 erg/cm
3deg
3⁄2, and other terms are found to be negligibly small. This small value of the term
T2 can be expected from the present model. Experimental values of the magnetization derivative of
K1 at a constant field are found to be much larger than those at a constant temperature, and this fact can also be explained by the present model.
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Tatsumi Hioki, Yoshika Masuda
1977Volume 43Issue 4 Pages
1200-1206
Published: October 15, 1977
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Nuclear magnetic resonance and nuclear spin-lattice relaxation of
45Sc in an itinerant-electron ferromagnet Sc
3In have been studied in both ferro- and paramagnetic states. The temperature dependences of the Knight shifts and susceptibilities give the hyperfine field due to d-spin of +58.4kOe per Bohr magneton per Sc atom suggesting strong s-d admixture in the wave function at the Fermi surface and the d-spin contribution to the susceptibility. The external field dependence of the internal field at
45Sc has been measured and analyzed in terms of the hyperfine fields proportional to d-spin moment and the external field. The observed magnetic field dependence of (
T1T)
−1 in both states is explained very well by the self-consistent renormalization theory of spin fluctuations in which the effect of magnetic field was taken into account, in conjunction with the negative magnetoresistance measured by us.
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Masahiro Matsumura, Kunisuke Asayama
1977Volume 43Issue 4 Pages
1207-1215
Published: October 15, 1977
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The nuclear magnetic relaxation of
59Co in dilute Cr
1−xV
xCo (
x\lesssim0.05) and Cr
1−xMo
xCo (
x\lesssim0.25) alloys in the ordered state was investigated.
T1 is proportional to 1⁄
T in the region of
T<<
TN.
T1T decreases rapidly with the decrease of the ordering temperature associated with the increase of
x. This decrease of
T1T with the decrease of the ordering temperature is generally observed in randomly ordered systems in metals irrespective of the ferro and antiferromagnet. Approximate model calculations based on the Weger mechanism, where the nuclear Zeeman energy relaxes to the kinetic energy of the conduction electrons via the virtual excitation of the spin waves, have been carried out in PdCo, whose
T1 was already measured, and in CrVCo alloys. The experimental results are explained qualitatively well by the Weger mechanism.
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Shigeyuki Murayama, Hiroshi Nagasawa
1977Volume 43Issue 4 Pages
1216-1223
Published: October 15, 1977
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The temperature dependence and the magnetic field dependence of the resistivity of polycrystalline α-Mn metal were measured between 1.3 and 20 K in external transverse and longitudinal magnetic fields of up to 100 kOe. The anomalously large coefficient of the T
2 term in the low-temperature resistivity of α-Mn was found to decrease appreciably for increase in the applied magnetic fields. These results are interpreted in terms of the suppression of spin fluctuations in the antiferromagnetic α-Mn by the high applied fields. The magnetic field dependence of the resistivity, which was corrected for the effect of cyclotron orbital motion, is shown to be a linear function of the applied fields.
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Hira Lal Kharoo, O. P. Gupta, M. P. Hemkar
1977Volume 43Issue 4 Pages
1224-1228
Published: October 15, 1977
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The Grüneisen parameters of alkali metals (Li, Na, K & Rb) have been computed at various temperatures from the experimental and the recent theoretical values of the pressure dependence of the elastic constants, using an improved CGW model for their lattice dynamics. The computation is carried out by a modified Houston’s method in which the integral is evaluated by a six term approximation. The Grüneisen parameters calculated in our present study show reasonably satisfactory agreement with experimental observations.
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Nobuhiro Shiotani, Takuya Okada, Hisashi Sekizawa, Shinya Wakoh, Yasun ...
1977Volume 43Issue 4 Pages
1229-1236
Published: October 15, 1977
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Angular correlation of positron annihilation radiation in Cr and Mo were measured. Self-consistent band structure calculations for Mo were carried out by the APW method with state-dependent potentials. Theoretical angular correlations for Cr and Mo were also calculated by the APW method. Observed fine structures on the angular correlations and the crystalline anisotropies were well reproduced by the calculations. However, when the theoretical and experimental correlation curves were normalized to an equal area, the theoretical curves were consistently lower in counting rate than the experimental ones in small angle region, and higher in large angle region. This type of discrepancy between the theory and the experiment is the same as we previously found in V and Nb, and is ascribed to the electron-positron correlation effects.
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Takeshi Inoshita, Kenji Nakao, Hiroshi Kamimura
1977Volume 43Issue 4 Pages
1237-1243
Published: October 15, 1977
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The electronic band structure of the first-stage potassium-graphite intercalation compound C
8K was calculated by a semi-empirical tight-binding scheme. The calculated Fermi surfaces can be classified into two distinct types. One is potassium-like and nearly isotropic; the other is carbon-like and of cylindrical shape. In addition, the cylindrical portions show nesting property, which is likely to induce charge-density-wave instability. The isotropic portions of the Fermi surfaces are responsible for the large reduction of anisotropy in conductivity of C
8K relative to graphite. The calculated density of states has a peak around the Fermi level and is in good agreement with the observed density of states derived from the specific heat measurements.
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J. G. Mclarnon, D. Ll. Williams
1977Volume 43Issue 4 Pages
1244-1246
Published: October 15, 1977
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A point detector geometry with a resolution of 0.7 mrad. by 1.1 mrad. has been used to study the Fermi surface for several α phase alloys of
CuGe. The variation of the [111] neck diameter and the [110] Fermi radius has been determined as a function of germanium concentration. Comparisons are made with previous work on this and other copper alloy systems, and also with the rigid band predictions.
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Eiji Hashimoto, Satoru Kabemoto, Takao Kino
1977Volume 43Issue 4 Pages
1247-1254
Published: October 15, 1977
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Annealing profiles of vacancies in zone-refined aluminum were studied by electrical resistance measurement after quenching, and discussed under either assumption of uniform distribution of dislocations or non-uniform one. The annealing curves calculated for the non-uniform distribution of dislocations, using
Em1=0.65 eV,
Em2=0.50 eV and
B2=0.17 eV, show the excellent fit to the experimental annealing curves. It is suggested from such an analysis that the annealing experiment should be made on the specimen with a controlled dislocation density and configuration in order to clarify the fundamental properties of point defects in metals.
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Kouichi Ichikawa, Hiroo Nakamori, Kenjiro Tsutsumi, Takeshi Watanabe
1977Volume 43Issue 4 Pages
1255-1257
Published: October 15, 1977
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The Ti
Kβ X-ray spectra of metallic titanium and its oxides the precisely measured with a two-crystal spectrometer. It is found that the Ti
Kβ
1,3 line width is strongly affected by the oxygen concentration. The behavior is interpreted as being due to the interaction between 3
d electrons and a 3
p hole produced upon emission of the
Kβ
1,3 radiation. Also, the screening effect of 4
s conduction electrons seems to play an important role in reducing the width at relatively low oxygen concentration.
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Yoshio Waseda, Shigeru Tamaki
1977Volume 43Issue 4 Pages
1258-1261
Published: October 15, 1977
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The structure of liquid Au–Co alloys with 10, 20, 27, 30, 35 and 40 at% Co has been examined by X-ray diffraction. The shape of all these structure factors is very close to that of liquid gold and no additional peak and deformation in the structure factor
S(
Q) were confirmed. The temperature dependence of
S(
Q) for liquid Au-27 at% Co alloy has been also carefully investigated at six temperatures above the melting point and no anomalous behaviour was observed.
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Masaki Taniguchi, Shin-ichiro Narita
1977Volume 43Issue 4 Pages
1262-1269
Published: October 15, 1977
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Isolated
D− states in Sb-and As-doped germanium crystals have been studied by means of long-wavelength (submillimeter plus millimeter) photoconductivity measurements with a lamellar grating Fourier transform spectrometer at an extremely low temperature, 0.38 K. The electron binding energies of the isolated
D− states are accurately determined and the shift of the
D− state energy is clearly observed between the samples with different impurities. The many valley effect of the conduction band on the
D− state energy is confirmed by comparing the spectra under high [111] stress with those of stress free. The energy shemes of the
D− states in Sb-and As-doped germanium crystals are clarified.
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Akiko Natori, Hiroshi Kamimura
1977Volume 43Issue 4 Pages
1270-1279
Published: October 15, 1977
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The binding energies of a D
− ion in the stress free and high stress cases are calculated with use of the Chandrasekhar type variational function. In the approximation of neglecting the valley-orbit interaction, the ionization energy of an electron from a D
− ground state to a conduction band in the intravalley electron configuration corresponds to the D
− binding energy in the high stress case while that in the intervalley configuration to the binding energy in the stress free case. In the former case the calculated value is the half of the observed one while in the latter case the calculated value is in fair agreement with the observed one. The energy difference between two cases is mainly due to the difference between the intra-and inter-valley Coulomb interactions.
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Jun-ichiro Kanbe, Hideo Onuki, Ryumyo Onaka
1977Volume 43Issue 4 Pages
1280-1285
Published: October 15, 1977
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The photoelectron spectra of PbCl
2, PbBr
2 and SnCl
2, which have the lead chloride-type crystal structure, have been measured with X-rays and extreme ultraviolet rays in order to investigate the electronic structures of their valence bands. The photoelectron spectra of TlCl and Pbl
2 have also been measured for comparison because they have the same electronic configuration as PbCl
2 et al. though the crystal structures are different. It was found that the spectra of all above materials have a common feature, namely, the bands observed in the valence region consist of two parts, the lower binding energy band being much more intense than the other, and it further splits into three. It has been concluded that the higher part of the valence band of these crystals (the lower binding energy band) is mainly composed of
p electrons of halogen ions but considerable admixing of metal
s electrons is present.
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Atsuko Sumi
1977Volume 43Issue 4 Pages
1286-1294
Published: October 15, 1977
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It is shown that an electron and a hole interacting mutually through the Coulomb force in the acoustic-phonon field take, within the adiabatic approximation, four possible phases depending upon the coupling constants: the lowest state is the free exciton in phase[I], the large-radius self-trapped exciton in [II], the small-radius self-trapped exciton in [III
+], and a pair of self-trapped electron and self-trapped hole in [III
−]. The center-of-mass motion of exciton changes discontinuously to be self-trapped as one moves from [I] to [II] or [III
+] with increase in the phonon-coupling constants. The relative motion of exciton changes discontinuously to be self-shrinked as one moves from [I] or [II] to [III
+]. [III
+] and [III
−] are realized respectively for the same and opposite sign of the deformation potentials of electron and hole. When the Coulomb interaction energy is so large as to be comparable to the electron and hole band widths, discontinuous boundary between [II] and [III
+] disappears.
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Nobukata Nagasawa, Tsuneyoshi Mita, Tadashi Itoh, Masayasu Ueta
1977Volume 43Issue 4 Pages
1295-1300
Published: October 15, 1977
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Forward Raman scattering of excitonic molecule in CuCl has been studied at the giant two-photon excitation with using laser light having a wave vector
K0 but three different half band-widths, 0.2, 1.4 and 2.5 meV. In cases of laser excitation with broader half band-widths, the Raman and luminescence processes coexist and give emission lines called (LEP)
R and (LEP)
B, respectively. Both lines show the similar dependence of energy change upon the scattering angle. The (LEP)
R and (LEP)
B lines show red and blue shift, respectively, with the increase of laser excitation intensity. The excitonic molecule-state generated at
K=2
K0 is responsible for the (LEP)
R line, while the (LEP)
B line is considered to arise from a state having a certain
K value smaller than 2
K0. Excitonic molecules generated coherently by the giant two-photon excitation are assumed to relax towards
K=0 with keeping their individual momentum at almost the same value.
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Kêitsiro Aizu
1977Volume 43Issue 4 Pages
1301-1307
Published: October 15, 1977
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Following a previous paper, the present paper also investigates incommensurate modulation in K
2SeO
4. While the direction of modulation previously was assumed ⁄⁄
x, it presently is assumed ⊥
x. Directions ⊥
x are represented by the
y axis for simplicity’s sake. In view of the number of equivalent wavevectors, the transition parameter system adopted for the
x axis cannot be entirely analogous to that to be adopted for
y; this new system is determined. The thermodynamic potential function is found. A certain number of possible ferroic phases are deduced, which include phases incommensurate along one or both of the
x and
y axes. The problem “To which of these ferroic phases should the prototypic phase change if the transition is assumed second order?” is solved.
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Ryuji Abe, Noriyoshi Shibata
1977Volume 43Issue 4 Pages
1308-1313
Published: October 15, 1977
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The behaviours of two kinds of radicals, NH
3+(α) and NH
3+(β) in the γ-irradiated ammonium sulfate crystals were examined in more detail. Above
Tc each radical flipped between two stable configurations around the
a–
b plane with the frequency higher than 10
8 sec
−1, but below
Tc it tilted from the
a–
b plane with a certain angle. One half of the flipping angle was two or three times as large as the tilt angle. Based on the results a microscopic model for the ferroelectric phase transition of ammonium sulfate was considered. In the model it was assumed that at
Tc the SO
42− tetrahedron was newly deformed owing to the correlated movement in the NH
4+(α)–SO
42−–NH
4+(β) bonding and an abrupt increase of the dipole-dipole interaction energy occured. The small Curie constant of ammonium sulfate can then be explained satisfactorily by the model.
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Susumu Shiozaki, Akikatsu Sawada, Yoshihiro Ishibashi, Yutaka Takagi
1977Volume 43Issue 4 Pages
1314-1319
Published: October 15, 1977
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It is shown that (011) and (031) twin planes can be introduced in the orthorhombic phase of K
2SO
4 and K
2SeO
4, and both twin planes can be moved smoothly through crystals by appropriate external stress in the temperature range from about 300°C to the orthorhombic-hexagonal phase transition point. It is inferred from the crystal structure in the orthorhombic phase that SO
4−− (or SeO
4−−) radicals must have two stable states (the up and down states), and change from one state to another during the passage of twin planes. It is suggested that the space group of the hexagonal phase is D
6h4–P6
3/mmc, and the hexagonal-orthorhombic phase transition is essentially due to the ordering of SO
4−− (or SeO
4−−) radicals.
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Kiyoyasu Imai
1977Volume 43Issue 4 Pages
1320-1326
Published: October 15, 1977
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Precise dilatometric measurements of TGS revealed an existence of a distinct departure in the coefficients β
2 of thermal expansion from the mean field theory (MFT). In the reduced temperature range, −3.17<log
10−
t<−1.87, the data of β
2 fit well to the formulas given by a connection between the Larkin-Khmel’nitskii theory (LKT) and the Pippard relations. The fitted formulas explain satisfactorily also the behavior above
Tc, except for the close vicinity of
Tc considered as the region of ‘rounding’. In the wide range, 80 K to 321 K, a good agreement with the MFT is obtained by taking suitable parameters. The jump
Δβ
2 derived from the MFT-fit is comparable with the corresponding value in the LKT. A comparison between the results of TGS and dipolar Ising ferromagnet LiTbF
4 was made.
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Tomoyuki Hikita, Hiroshi Sekiguchi, Takuro Ikeda
1977Volume 43Issue 4 Pages
1327-1331
Published: October 15, 1977
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Dielectric properties were studied on fourteen langbeinite-type crystals. Measurements were performed in the temperature range 20∼−196°C for single or polycrystalline samples. It was newly found that five crystals undergo phase transitions; (NH
4)
2Mg
2(SO
4)
3 at −52°C, (NH
4)
2Ni
2(SO
4)
3 at −113°C, K
2Co
2(SO
4)
3 at −147°C, (NH
4)
2Ca
2(SO
4)
3 at −115°C and Rb
2Ca
2(SO
4)
3 at −90°C. A tentative discussion is made to classify the bahaviors of phase transitions in langbeinite family in respect to the lattice constants and ionic radii of constituent ions.
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Osamu Aono, Yoshishige Katayama
1977Volume 43Issue 4 Pages
1332-1336
Published: October 15, 1977
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A nonlocal phenomenological equation is introduced for a multicomponent fluid where chemical or nuclear reactions are taking place. The reciprocity between the nonlocal linearcoefficients is examined closely. An approximation reduces the nonlocal equation to the ordinary phenomenological relation with correction terms which show clearly a coupling of the reaction with the diffusion and the thermal conduction in an isotropic system.
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Kozo Hoshino, Mitsuo Watabe
1977Volume 43Issue 4 Pages
1337-1341
Published: October 15, 1977
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The electrical conductivity is calculated in the single-bond coherent-potential approximation for the electrons in the disordered lattice with only the fluctuation of transfer energy. The results are discussed in connection with the behaviour of the mobility edge, determined recently by Economou and Antoniou, as a function of the magnitude of fluctuation of transfer energy.
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Yoshinori Takahashi
1977Volume 43Issue 4 Pages
1342-1350
Published: October 15, 1977
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Dissociative chemisorption process of a molecule on a metal surface is discussed through the Anderson model. The density of states, the bond order, and the potential energy curve are calculated for various values of molecule-metal coupling constants.
A qualitative explanation is given for the reason why the activation energy of H
2-dissociation is larger on a Cu surface than on a Ni surface.
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Takeshi Noro, Kiyoshi Tanaka, Kimio Ohno
1977Volume 43Issue 4 Pages
1351-1357
Published: October 15, 1977
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For the
B1Σu+ and
b3Σu+ states of the H
2 molecule, CI calculations are carried out using a small basis. The mixing of Rydberg and valence-shell characters in these states is analyzed for a wide range of internuclear distance (1.4 a.u.≤
R≤10 a.u.). The
B1Σu+ state shows a complicated
R dependence. It is Rydberg type in small
R(1.4 a.u.≤
R≤2.44 a.u.), a heavy mixture of valence-shell type and Rydberg type for intermediate region (2.44 a.u.<
R<6.0 a.u.), and Rydberg type for large
R(
R≤6.0 a.u.). The
b3Σu+ state, on the other hand, changes rapidly from Rydberg type to valence-shell type at
R=2.0 a.u. when
R increases. During the course of the above analysis an index to the degree of the mixing is found. This index would be useful in discussion about Rydberg and valence-shell characters.
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Shoichi Kai, Kenji Matsuo, Kazuyoshi Hirakawa
1977Volume 43Issue 4 Pages
1358-1360
Published: October 15, 1977
Released on J-STAGE: May 29, 2007
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Several patterns are observed in the electrohydrodynamic instability of binary mixtures of nematic and cholesteric liquid crystals. The phase diagrams are obtained for the composition and frequency.
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S. C. Srivastava, M. S. Sinha
1977Volume 43Issue 4 Pages
1361-1363
Published: October 15, 1977
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The dielectric constant and dielectric loss of ethyl trichloroacetate in non-polar solvents were measured at eight microwave frequencies at 25°C. In cyclohexane and p-xylene solutions, the Cole-Cole plots for ethyltrichloroacetate were symmetrical, but the plot was unsymmetrical in p-dioxane solution. The data were also analysed using two relaxation times τ
1 and τ
2, which were associated with the overall and group relaxation processes of molecules, respectively. The overall relaxation time τ
1 increased in the solvent order; cyclohexane<p-xylene<p-dioxane. This fact indicates that the solute-solvent interaction, mainly the dipole-induced dipole interaction, increases in the solvent order.
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Yasushi Nishida, Shuichiro Kawamata, Kazushige Ishii
1977Volume 43Issue 4 Pages
1364-1370
Published: October 15, 1977
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The electrostatic ion stoppering in a magnetic mirror field is demonstrated experimentally in rather high plasma density (10
10<
n0\lesssim10
13cm
−3). The ion loss from the mirror throat expressed by a loss factor δ, is reduced to about one quarter of the initial value. It is discussed as a confinement mechanism of ions that particles are reflected back adiabatically by the electrostatic field at the mirror throats of the magnetic field.
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Tatsuki Ogino, Susumu Takeda
1977Volume 43Issue 4 Pages
1371-1377
Published: October 15, 1977
Released on J-STAGE: June 01, 2007
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The fast magnetosonic waves in cylindrical and inhomogeneous plasmas propagating towards the axis are studied by a computer simulation and a theoretical analysis. The velocity and amplitude of the wave excited by a magnetic field perturbation increase due to the cylindrical and nonlinear effects.
The propagation characteristics of the fast magnetosonic waves depend on σ
2⁄2, the ratio of amplitude to the square of frequency. The large amplitude soliton-like pulses are efficiently excited for 1\lesssimσ
2\lesssim100 by a positive half cycle of a sinusoidal wave. The wave packets are produced for σ
2\gtrsim1 by a sinusoidal perturbation.
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Reiji Sugaya, Masao Sugawa, Hisayuki Nomoto
1977Volume 43Issue 4 Pages
1378-1384
Published: October 15, 1977
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The instabilities of electron cyclotron harmonic waves due to the anisotropy of the electron velocity distribution produced by the injection of the electron beam perpendicular to the magnetic field. A strong spontaneous emission growing up 60 dB above background noise appears near the electron cyclotron harmonics. This instability cannot be launched or sychronized by external modulation. The amplitude is usually not steady in time, but switches off and on in time intervals of 10∼100 μsec. It grows exponentially in time initially, saturates and disappears. This instability can be explained by dispersion relations of electron cyclotron harmonic waves propagating perpendicular to the magnetic field in a plasma with a mixture of ring and Maxwellian electron distributions. The measured growth rate is smaller by 2 to 5 times than the theoretical ones.
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Yoshiro Nakagawa, S. S. Medley
1977Volume 43Issue 4 Pages
1385-1392
Published: October 15, 1977
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Ion heating by the strong current in the Texas Turbulent Torus has been investigated with the charge exchange fast neutral measurement with respect to correlation with a current penetration into the plasma column. At relatively low density (
n≅2×10
12 cm
−3), the number of heated ions increases as the current penetrates into the central region of plasma column until the current peak (
t≅1.5 μsec). Ion energy distribution function is Bi-Maxwellian and bulk ions are heated up to temperature in excess of 300 eV at about 200 nsec from the start of heating current. Temperature of the high energy tail, of which population is several % of total ions, increases to a maximum temperature of 3.5 keV at 0.8 μsec. At high density (
n≅7×10
12 cm
−3), temporal evolution of radial distribution of heated ions shows that energetic ion production is restricted within the skin current region during 1.5 μsec.
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Kazuhiro Nozaki, Katsunobu Nishihara
1977Volume 43Issue 4 Pages
1393-1399
Published: October 15, 1977
Released on J-STAGE: June 01, 2007
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It is shown by computer simulations that a diverging thermonuclear reaction wave in a high density plasma is an accelerating overcompressed detonation. The propagation stages of the reaction wave are classified according to different processes of energy transfer such as the α-particle diffusion, the shock heating and the electron thermal conduction. The front of the reaction wave consists of the shock compressed region proceeded by a pre-heating zone, where the effect of α-particle diffusion exceeds that of the electron thermal conduction.
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Hideo Sugai, Shunichi Hirose, Susumu Takeda
1977Volume 43Issue 4 Pages
1400-1406
Published: October 15, 1977
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In a weakly ionized plasma with a perpendicular electric field
E⊥ and an axial magnetic field B, ion temperature has been observed to be approximately proportional to (
E⊥⁄
B)
2. The observed ion heating is well explained by simple calculations based on a Joule heating which is caused by
E×
B drift.
The transient process of the heating is also investigated in a pulsed experiment, a loss of the initial cold ions and a slow production of hot ions have been observed.
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Takasi Tuda, Masatoshi Tanaka
1977Volume 43Issue 4 Pages
1407-1410
Published: October 15, 1977
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A new type of impurity drift instability is studied in the limit of short mean free path. The mode is driven by the ion parallel viscosity, and is stabilized by the collisional diffusion across the magnetic field when the impurity concentration is less than a certain value. This coincides with the stability condition for the collisionless impurity drift mode.
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Hitoshi Hojo, Hiromichi Tabuchi, Kyoji Nishikawa
1977Volume 43Issue 4 Pages
1411-1416
Published: October 15, 1977
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Three-dimensional nonlinear Schrödinger equation for an electrostatic ion cyclotron wave coupled to an ion acoustic wave is derived with the use of the reductive perturbation method. Electrons are assumed to obey the Boltzmann law under the influence of the electrostatic potential. Cold fluid equations are used for the ions. Instability of a plane electrostatic ion cyclotron wave against a two-dimensional modulation is investigated and the unstable regions are graphically plotted in the wavenumber space.
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Akira Yoshizawa
1977Volume 43Issue 4 Pages
1417-1423
Published: October 15, 1977
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A statistical-mechanical analysis is made of Kolmogoroff’s−5⁄3 power law in the inertial subrange of turbulent field. This paper proposes a method of removing the divergence of the response equation at low wave numbers, which is caused by the convection of small eddies by big ones and is a stumbling block to the analytical derivation of Kolmogoroff’s spectrum. Results obtained are in good agreement with the experimental value of Kolmogoroff’s constant.
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Ryogo Hirota
1977Volume 43Issue 4 Pages
1424-1433
Published: October 15, 1977
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A systematic method for isolating certain nonlinear partial difference equations that exhibit solitons is proposed. A nonlinear partial difference equation which approximates the Korteweg-de Vries equation in the weakly nonlinear and continuum limit, is obtained. N-soliton solutions, the Bäcklund transformation and the inverse scattering transform for this equation are presented.
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Yoshimoto Onishi
1977Volume 43Issue 4 Pages
1434-1440
Published: October 15, 1977
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The behavior of a slightly rarefied vapor gas flowing around its spherical condensed phase is investigated on the basis of the linearized BKW (or BGK) equation and the diffuse reflection boundary condition.
It is shown that the pressure field induced by velocity field plays an important role. The condensation occurs over the front part of the condensed phase and the evaporation over the rear due to this pressure field. This interphase transfer process reduces the total drag acting on the spherical condensed phase.
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Akira Noguchi, Hideaki Watanabe, Kiyoshi Sakai
1977Volume 43Issue 4 Pages
1441-1446
Published: October 15, 1977
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The nonlinear self-dual network equation is exactly solved by the inverse scattering method. The equation is the discrete version of the modified Korteweg-de Vries equation with negative dispersion coefficient. Considerating the integral on the Riemann surface, the Gel’fant Levitan (Marchenko) equation is obtained. Soliton and shock wave solutions with non-zero asymptotic values are given.
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