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J. M. Saviron, D. González, J. L. Brun, J. A. Madariaga
1975 Volume 39 Issue 6 Pages
1417-1421
Published: December 15, 1975
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Analytical expressions for the non steady separation factor of an isotopic multicomponent mixture in a thermal diffusion column are given. The results, which are appropiate for column operation at total reflux and cover the real case in which small non active end volumes are present, show a simple exponential rising of the logarithm of the reduced separation factor independent of the initial mixture composition. This fact is confirmed by experimental transient data previously reported by Brun
et al. and by new experimental work presented here.
It is shown that the relative variations of the relaxation time with the hot wire temperature and with the operation pressure are just those predicted by the Furry, Jones and Onsager theory. It is concluded that two experimental operations: steady-separation vs pressure and non-steady separation vs time, and the use of FJO theory will allow us the qualitative prediction of the column operation in the usual temperature and pressure range in laboratory operation
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Kêitsiro Aizu
1975 Volume 39 Issue 6 Pages
1422-1430
Published: December 15, 1975
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Of homophone systems of phase transitions, especially those in which the soft modes are doubly degenerate are investigated in a general and unified way upon the basis of the considerations in the preceding paper [K. Aizu: J. Phys. Soc. Japan
38 (1975) 1592]. It is found that three general forms are possible for their
pedigrees. It is clarified what character of the prototypic phase and the soft modes are responsible for this essential differentiation of pedigrees. The number of all situations of a ferroic phase of each
rank in each general pedigree is determined. Illustrations are carried out with some cases where the space group of the prototypic phase and the transformation property of the soft modes are specified.
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Nobuhiko Saitô, Naoteru Hirotomi, Atsushi Ichimura
1975 Volume 39 Issue 6 Pages
1431-1438
Published: December 15, 1975
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It is shown that the induction phenomenon in the exchange of energies of normal modes found by computer experiments is an inherent property of the anharmonic lattice vibration and its behavior obeys the time reversal even after the elapse of the induction period. The instability of the normal modes when one mode is excited initially is related to the induction phenomenon, and is discussed by the application of the instability region of the Mathieu function. The exponential orbital separation is also shown to take place after the elapse of the induction period. This guarantees the C-property of the anharmonic lattice vibration.
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Hidetoshi Fukuyama, Toshio Tsuzuki, Sadao Nakajima
1975 Volume 39 Issue 6 Pages
1439-1442
Published: December 15, 1975
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Dimensionality of the density fluctuation of electron-hole systems in strong magnetic fields is examined in connection with the possibility of the excitonic phase. Our system consists of one conduction and one valence band. Even in extremely strong fields where only one Landau level of each carrier is taken into consideration and the energy spectrum is purely one-dimensional, the density fluctuations are three-dimensional as far as magnetic field strength is finite. This is due to the motion of carriers which is perpendicular to the field and caused by interactions. Thus the phase transition with the excitonic order parameter may occur at a finite temperature. However, as the field is increased, fluctuations acquire one-dimensional characteristics and critical temperature should be reduced.
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Tsuneharu Takeda, Tadao Kasuya
1975 Volume 39 Issue 6 Pages
1443-1453
Published: December 15, 1975
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In a ferromagnetic semiconductor with a narrow band the mechanism which causes magnetization of localized spins around a conduction electron is similar to that of the double exchange interaction, and the potential which traps the conduction electron is a pseudopotential. It is shown that the spin flip processes of the conduction electron make the magnetic polaron unstable, and that even in the case of the narrow band limit the radius of the magnetic polaron is large extending over many lattice sites. These properties are different from those of the usual lattice polaron in narrow band.
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Masanori Sugahara
1975 Volume 39 Issue 6 Pages
1454-1461
Published: December 15, 1975
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Basing on the time-dependent Ginzburg-Landau theory, we investigate the current-induced-transition state of type II superconductors in longitudinal magnetic field. A new mixed state in space-time domain is found, where the time integral of voltage difference is quantized in flux quantum. Experimentally observed transition properties in Pb films are explained with the help of the theoretical investigation. Interference patterns appeared in current-voltage curves give a conclusive evidence of the new mixed state in the transition state of superconductors.
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Masahiro Hirano, Shinichi Nakamura, Tachiro Tsushima
1975 Volume 39 Issue 6 Pages
1462-1466
Published: December 15, 1975
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Annealing behavior of magnetic anisotropy in LPE garnet films are investigated. There exists a good correlation between the activation energy for the decreasing process of
Ku and the difference between the ionic radii of the constituent rare earth ions. It implies that this difference is the physical origin for the nonuniform distribution of the rare earth ions which results in the presence of the uniaxial anisotropy. Further, the anisotropy with cubic symmetry is enhanced by the nonuniform distribution.
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Masatoshi Sato, Kinshiro Hirakawa
1975 Volume 39 Issue 6 Pages
1467-1472
Published: December 15, 1975
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The surface magnetization of Ni fine particles has been measured by the small angle scattering of polarized neutrons. It is pointed out that the θ dependence of the flipping ratio
R(θ) scattered at small angles θ is very sensitive to the existence of anomalous magnetic surface layers but insensitive to the existence of particle-particle spacial correlations. Beside these, the scattering cross section is extremely high, encouraging us to study the surface state by neutron scattering. Based on the informations of the radius of Ni and the thickness of the NiO coverage obtained from X-ray diffraction, a model is proposed so as to get a best fit to the observed
R(θ). According to this model, there exists about 3∼4 magnetic dead layers or 2 layers of reversed magnetization at the Ni surface.
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Katsukuni Yoshida
1975 Volume 39 Issue 6 Pages
1473-1481
Published: December 15, 1975
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Anomalous electric fields which have been observed in bismuth and antimony in high magnetic fields at low temperatures are investigated with particular reference to specimen size. The anomalous fields, contrary to the usual magnetoresistance, appear in the form of dip and hump in the angular-dependence diagram of the potential difference which is measured at a side surface of specimen. Since the dip and hump are strongly affected by geometrical conditions such as specimen size and location of current electrodes, the anomalous electric fields are considered to originate from the inhomogeneous current distribution, which is expected when the cross-section of specimen is large compared with the contact area of current electrodes.
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Yositaka Onodera
1975 Volume 39 Issue 6 Pages
1482-1485
Published: December 15, 1975
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The singularity of the
L2,3 X-ray absorption edge of light metals possesses a doublet structure owing to the spin-orbit splitting of the core
p level. The observed intensity ratio of the doublet is deviated from the expected 2:1. The deviation can be explained by introducing the electron-hole exchange scattering. A line shape formula is obtained which takes account of the exchange and spin-orbit interactions. It is used to analyse the Na spectra with success.
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Tsunekazu Matsuyama, Masahiro Saidoh, Noriaki Itoh
1975 Volume 39 Issue 6 Pages
1486-1491
Published: December 15, 1975
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The optical absorption bands associated with the
d10(
1S)→
d9s(
1D,
3D) transitions of Ag
+ in CsBr are studied. The area under the absorption curve decreases with increasing temperature from 10 K to room temperature, indicating that the Ag
+ ion in CsBr is in a deep off-center potential. Ten optical absorption bands are identified and these are ascribed to the transitions from the
d10 multiplets to the
d9s multiplets split in a C
3v symmetry. Good agreement between the experimental and calculated transition energies are obtained, although the poor agreement has been reported for alkali halides with NaCl-structure. This results is discussed in terms of the molecular orbital formation between the Ag
+ ion and neighboring halogens.
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Seiichiro Ikehata, Wataru Sasaki, Shun-ichi Kobayashi
1975 Volume 39 Issue 6 Pages
1492-1497
Published: December 15, 1975
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Spin echo spectra, Knight shift and spin-lattice relaxation time are measured on
31P in silicon crystals with phosphorus concentrations ranging from 4.5×10
18cm
−3 to 9.6×10
19cm
−3 over a temperature region from 4.2 K to 0.4 K. The shift and width of
31P line is atrributed to the inhomogeneous electron contact field. The results together with those of
29Si (J. Phys. Soc. Japan
36 (1974) 1377) support the Mott transition mechanism of metal-non metal transition and allow to interpret various properties of the metallic samples in terms of an electron gas with correlation.
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Takehisa Yoshinari, Masamitsu Hirai
1975 Volume 39 Issue 6 Pages
1498-1505
Published: December 15, 1975
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It has been confirmed that KI and RbI crystals under the two-photon excitation by a dye laser exhibit three emission bands at 3.05 eV, 3.31 eV, 4.10 eV and 2.27 eV, 3.12 eV, 3.96 eV, respectively, which are the same as those under the conventional one-photon excitation at low temperature. The intensity of the 3.05 eV and 3.31 eV emissions in KI decay with respective two decay times. The fast and slow components of these emissions exhibit almost identical emission spectra with the half width of 0.33±0.03 eV. The 2.27 eV and 3.12 eV emissions in RbI decay also by the fast and slow decay times. Temperature dependence of the decay time and intensity of these emissions has been studied, and possible electronic states responsible for these emissions are discussed.
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Eiichi Hanamura
1975 Volume 39 Issue 6 Pages
1506-1515
Published: December 15, 1975
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The electronic structure of excitonic molecule is discussed by taking into account the detailed band structure of CuCl, CuBr, CdS, CdSe and ZnO. Especially the excitonic molecule in CuBr is interesting due to the less simple valence band. The fine structure of the excitonic molecule is clarified under the effective electron-hole exchange effect and the interband hole-hole scattering beyond the effective mass approximation.
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Eiichi Hanamura
1975 Volume 39 Issue 6 Pages
1516-1524
Published: December 15, 1975
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The optical properties of the excitonic molecule are clarified, basing upon the electronic structure of the excitonic molecule derived in the preceding paper. The luminescence, the optical conversion of a single exciton into the excitonic molecule and the giant two-photon absorption due to the excitonic molecules are theoretically discussed and compared with the available experimental data.
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Yoshihiro Ishibashi, Yutaka Takagi
1975 Volume 39 Issue 6 Pages
1525-1528
Published: December 15, 1975
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The electrostrictions in KH
2PO
4 are discussed. It is shown that both the spontaneous strain in the ferroelectric phase and the field-induced strain in the paraelectric phase can be interpreted in a unified fashion even in terms of the simplest Slater model by taking into account the coupling between the strain and the fraction of sideway H
2PO
4− radicals,
r. The order parameter θ, previously introduced by other workers, may not be necessary for the explanation of the peculiar nateur of the electrostrictions in this material.
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Satoru Mashimo, Yasuo Iwasa, Akio Chiba, Kenichi Shinohara
1975 Volume 39 Issue 6 Pages
1529-1537
Published: December 15, 1975
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Dielectric transition similar to that found in poly(vinyl acetate) solution was also observed in dioxane solution of poly(vinyl chloride) and poly (
p-chlorostyrene) in carbon tetrachloride. It is shown that the dielectric dispersion observed above the transition temperature is attributed to a rotational motion only of a few monomeric units between two bonds undergoing rotation. On the other hand, below the transition temperature, the chain motion is subject to restriction caused by some intrachain interaction and a large number of the monomeric units must move together because of that interaction. Measurements of the intrinsic viscosity on poly(vinyl acetate) in carbon tetrachloride and poly(vinyl chloride) in dioxane show that the transition is a conformational transition from a loosely coiled chain molecule to a compact chain molecule. It is shown that the transition is a kind of globule-coil transition suggested theoretically by some authors.
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Isamu Todo
1975 Volume 39 Issue 6 Pages
1538-1542
Published: December 15, 1975
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The temperature dependence of elastic stiffness constant C
22 and ultrasound velocity of TGSe single crystals have been measured accurately near the ferroelectric phase transition. It is found that the anomalous part of the elastic stiffness constant
Δ C
22 and that of sound velocity are both proportional to log(
T−
Tc). The anomalous attenuation
Δα
1⁄2 in the paraelectric phase transition is also proportional to log(
T−
Tc).
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Koichi Matsuura, Ichiro Tsurumi
1975 Volume 39 Issue 6 Pages
1543-1546
Published: December 15, 1975
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Measurements of the conductivity and the Hall effect in high conductivity CdS crystals have been made at liquid nitrogen temperature, under the compressional uniaxial stress applied parallel or perpendicular to the
c-axis. It has been found that the change in the conductivity induced by the applied stress is substantially due to the change in the electron mobility. The mobility decreases with increasing the stress when the mobility under zero stress is near the intrinsic mobility, while the mobility increases with the stress when the mobility under zero stress is smaller than the intrinsic mobility. This behavior is explained in terms of the negative stress coefficient of the intrinsic mobility, (−2.9±0.5)×10
−11dyn
−1cm
2 and the positive coefficient of the extrinsic mobility, (2.7±0.3)×10
−10dyn
−1cm
2.
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Takehiko Ishiguro, Koji Kajimura, Seiichi Kagoshima, Hiroshi Tokumoto, ...
1975 Volume 39 Issue 6 Pages
1547-1557
Published: December 15, 1975
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Spike-like quantum oscillation is found in the absorption of longitudinal heat pulse propagating in Bi under magnetic fields. By comparing the period with that of the de Haas-van Alphen oscillation, we find that the electrons are concerned with the oscillation. Absorption of any phonon occurs only when the change in perpendicular component (to the magnetic field) of electron wave number accompanying the absorption is smaller than the inverse of the cyclotron radius. This fact allows the electron transition within a Landau level to occur only when the bottom of the Landau level is close to the Fermi level. This explains occurrence of spike-like oscillation even for the heat pulse with a broad frequency spectrum. The background comes from transition between different Landau levels. Concerning the transverse mode, the amplitude of the oscillation is smaller than the longitudinal mode by one order of magnitude.
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Hiroshi Maeta, Tadao Iwata, Shigeo Okuda
1975 Volume 39 Issue 6 Pages
1558-1565
Published: December 15, 1975
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Change in the
c-axis spacing in pyrolytic graphite after fast neutron irradiation at 5 K and subsequent isochronal pulse annealings have been measured in the range of 5∼900 K by X-ray diffraction method. The
c-axis expansion was estimated to be
Δc0⁄
c0=3.4
Ni, where
Ni is the fractional concentration of interstitial atoms. This corresponds to a volume change of 3.3 atomic volume per interstitial atom. For annealings of the
c-axis spacing, a small recovery below 80 K was followed by a large recovery at around 100 K, and above it a small continuous recovery occurred up to 900 K. The large recovery at around 100 K was interpreted by the formation of
C2 molecules and interstitial clusters. The present results were discussed comparing with the so far reported results of electrical resistivity, thermal resistivity and stored energy release measurements.
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Takayoshi Suzuki, Hyongyu Kim
1975 Volume 39 Issue 6 Pages
1566-1571
Published: December 15, 1975
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The temperature and strain-rate dependence of the critical resolved shear stress of LiF single crystals has been measured in the temperature range from 4.5 to 300K. The results are analysed on the basis of the thermally activated deformation process. The data below 20K are shown to correlate well with the requirements of the Peierls mechanism. The Peierls stress is deduced to be 2.0 kg/mm
2 when the parabolic Peierls potential is assumed, and 1.7
5 kg/mm
2 for the sinusoidal case. The estimated value of the activation energy is about 0.09 eV, which give a reasonable value for the line energy of a dislocation. The activation volumes determined by changes in strain rate also exhibit the proper trends for the Peierls mechanism.
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Masako Kajiura, Kiyoshi Aoyagi, Takahiko Tamaki
1975 Volume 39 Issue 6 Pages
1572-1578
Published: December 15, 1975
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Optical properties of
R-excitons in LuCrO
3 as well as their change during the magnetic-field-induced spin reorientation have been investigated. It is shown that the polarization characters of the exciton lines agree with the theory of the Frenkel excitons in antiferromagnetic rare-earth orthochromites. By using the available theory, parameters related to the excitation transfer matrix elements of Cr
3+ ions in LuCrO
3 are determined. The energy shift and intensity change of the exciton lines during the spin reorientation are discussed and compared with those in YCrO
3.
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Tadasu Suzuki, Hisao Nagasawa
1975 Volume 39 Issue 6 Pages
1579-1585
Published: December 15, 1975
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The angular dependence of the intensity of X-ray Raman scattering from polycrystalline beryllium and graphite has been studied using Cr
Kβ
1 and Cu
Kα radiations, respectively. At lower scattering angles the angular dependence of the peak intensity values of the Raman band is in good agreement with the theoretical curve deduced from the dipole approximation. A marked discrepancy, however, appeared at higher scattering angles. This discrepancy could be mitigated by an improved analysis which takes into account the multipole transitions. The expression obtained for the intensity of the X-ray Raman scattering is:
(
Remark: Graphics omitted.),
where “
a” denotes the mean radius of the charge distribution of the
K-electron of the scatterer elements,
T1(λ) and
T2(λ) are related with the dipole and multipole transitions, respectively.
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Yoshimi Tsuchiya, Seiichiro Noguchi, Tomoe Fukamachi, Sukeaki Hosoya
1975 Volume 39 Issue 6 Pages
1586-1589
Published: December 15, 1975
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Comption profile of ultra-fine particles of Cu was measured by the use of a solid state detector and
241Am isotope γ-ray source. The momentum distribution of electrons in such particles has been investigated in comparison with a polycrystalline Cu. The profile of these particles has proved to have an FWHM value narrower than that of the polycrystalline sample. The narrowing is mainly attributed to the surface state of electrons. The results were discussed in comparison with those by positron annihilation for the corresponding sample.
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Fumihiro Koike
1975 Volume 39 Issue 6 Pages
1590-1595
Published: December 15, 1975
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Theoretical investigations are made for elastic scattering and vibrational excitation via a vibrationally excited transient ionic state, following the reaction
e+
AB→
AB−**(υ′)→
AB(υ)+
e. Restrictions on the electronic wave number
k and on the resonant partial wave angular momentum
l are such that
k<<1 and
l≥1. A threshold law is proposed: a resonance width between the vibrational υ and υ′ states,
Γυυ′, is proportional to
k2l+1 multiplied by a square of the Franck-Condon factor
Fυυ′. This is an extention of the usual Wigner rule,
Γυυ′∝
k2l+1.
The results of semi-empirical calculations are presented for O
2 and NO. By using only one calibration parameter, satisfactory results are obtained. Resonance widths of the transient υ′ states and energy integrated vibrational excitation cross sections are calculated. For the life time of O
2−**(υ′=4), 7.2×10
−11sec is obtained. This value is consistent with all available experimental data.
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Masao Ushio, Tsutomu Ishimura
1975 Volume 39 Issue 6 Pages
1596-1602
Published: December 15, 1975
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The measurement of time development of plasma conductivity in a turbulent heating is done at various radial positions in a plasma by using an electric probe and a Rogowsky coil by which the quasi static electric field strength and current density are measured. In the early phase of the discharge, the plasma conductivity in the current penetrating domain shows anomalously low value ranging from 1.7 to 7 Ω
−1cm
−1, that is of the order of one tenth of one tenth of the classical one at 2 eV in electron temperature, despite that the overall voltage waveform does not show any resistive hump. After the full penetration of the current to the column axis the conductivity begins to drop rapidly at all radial points and the resistive hump of the overall voltage waveform begins to rise, and the macroscopic instability grows.
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Shoichi Wakiya
1975 Volume 39 Issue 6 Pages
1603-1607
Published: December 15, 1975
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The bipolar coordinate solution of the two-dimensional Stokes equations is applied to flows around two circular cylinders. It is proved that there are three cases which this kind of solutions can describe. Solutions are presented for a cylinder revolving eccentrically in a cylindrical frame, a cylinder in the neighborhood of a plane wall and two cylinders in rotary motion as a pair.
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Ri’ichi Matsuzaki
1975 Volume 39 Issue 6 Pages
1608-1613
Published: December 15, 1975
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The nonequilibrium flow properties behind a strong normal shock wave in the nitrogen gas are studied by using a set of equations which was developed previously by the author to be applied to a quasi-one-dimensional flow of a partially ionized nitrogen. Numerical solutions of this set of equations show some typical flow properties in nonequilibrium. The flow is not only in chemical nonequilibrium, but also in thermal nonequilibrium between electrons and heavy particles. Regardless of its initial values, the electron temperature is always lower than that of heavy particles.
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Katuro Sawada, Takeyasu Kotera
1975 Volume 39 Issue 6 Pages
1614-1618
Published: December 15, 1975
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Integrals of Hénon’s type are given for the system with inversely quadratic pair potentials. The explicit time dependence of solution are given for the repulsive case. A little extension and modification make it possible to have a solution for the system with quadratic and inversely quadratic pair potentials.
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Katsuhiko Nagano, Hisao Okamoto
1975 Volume 39 Issue 6 Pages
1619-1620
Published: December 15, 1975
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The sound attenuation constant is calculated for the one-dimensional ferromagnet. Its frequency and angular dependence turn out to be ω
k3⁄2 and cos
4θ, respectively. The effect of the uniaxial anisotropy is also taken into account in a self-consistent way.
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Masaaki Kaminaga
1975 Volume 39 Issue 6 Pages
1621-1622
Published: December 15, 1975
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New structures of voltage-current characteristics in Nb-Nb point contact Josephson junctions were found by using a differentiation technique. The first and the second derivatives of junction voltage with respect to the current as a function of bias reveal finer structures than
V–
I characteristics of junction. These new structures can be regarded as the result of thermal runaway of multiple point contacts in the Josephson junctions due to Joule heating. When one of the multiple point contacts suffers thermal runaway, the resistance of the junction changes suddenly and the peaks appear in
V–d
V⁄d
I and
V–d
2V⁄d
I2 characteristics.
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Yuji Ito, Akira Ohsawa
1975 Volume 39 Issue 6 Pages
1623-1624
Published: December 15, 1975
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Antiferromagnetic orbital ordering patterns of CoS
2 in which four Co atoms at fcc positions of pyrite structure have different orbital states are searched for using the polarized neutron diffraction technique. We concluded negative results on the antiferromagnetic orbital patterns investigated, with the four orbital states being all equal within the experimental accuracy.
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Munetaka Haida, Kay Kohn, Jinzo Kobayashi
1975 Volume 39 Issue 6 Pages
1625-1626
Published: December 15, 1975
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Measurements of magnetic torque and magnetoelectric susceptibility of CuCl boracite indicate that both weak ferromagnetic moment and spontaneous polarization are parallel to the [001] axis at 4.2 K and consequently its magnetic point group is m′m′2. The result indicates the existence of a new group of boracite where weak ferromagnetic and electric moments are parallel.
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Junji Mada, Shuichi Iida
1975 Volume 39 Issue 6 Pages
1627-1628
Published: December 15, 1975
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Mössbauer spectra of low temperature phase of Magnetite (Fe
3O
4) has been studied by changing θ(the cooling-field angle measured from [001] to [1\bar10] within the (110) plane). Data were analyzed for θ=0° and 40° cases with a computer and new assignments have been obtained.
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Tsuyoshi Murao
1975 Volume 39 Issue 6 Pages
1629-1630
Published: December 15, 1975
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Nuclear magnetic properties of the single crystal (paramagnetic) and the polycrystal (ordered) praseodymium metal are discussed by using the effective nuclear spin Hamiltonian recently derived by the author. The Hamiltonian can explain the anomalous nuclear specific heat of the single crystal praseodymium metal as well as the magnitude of the nuclear Curie temperature found in this crystal in a consistent way. Informations can also be obtained for the low-lying states of the 4f electrons.
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Shinji Kawaji, Shin-ichiro Miki, Takao Kinoshita
1975 Volume 39 Issue 6 Pages
1631-1632
Published: December 15, 1975
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Superconducting resistive transition is observed in
n-type inversion layers on
p-type InAs surfaces. The transition temperature is about 2.7 K. Overall behaviours are phenomenologically well explained by the theory of fluctuation effects in two-dimensional superconductors.
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Tsuyoshi Imai, Kiyoshi Yatsui
1975 Volume 39 Issue 6 Pages
1633-1634
Published: December 15, 1975
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An experimental study of parametric instability driven by a beam modulation near the lower hybrid frequency is presented. If the modulation voltage exceeds a threshold value, the pump wave appears to decay into an ion acoustic wave and a lower hybrid wave. The threshold electron drift speed is found to be of the order of the ion acoustic speed as predicted by a theory of parametric instability in an inhomogeneous plasma.
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Kazuaki Narita
1975 Volume 39 Issue 6 Pages
1635-1636
Published: December 15, 1975
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New classes of the differential-difference equations which lead to the Volterra system are presented and the special solutions of those equations are obtained.
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Toshihiko Shigematsu
1975 Volume 39 Issue 6 Pages
1636A
Published: December 15, 1975
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Koichi Matsuura, Toshio Honjo, Ichiro Tsurumi
1975 Volume 39 Issue 6 Pages
1636B
Published: December 15, 1975
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Yoshiro Irie, Mikio Hyakutake, Masaru Matoba, Masateru Sonoda
1975 Volume 39 Issue 6 Pages
1636C
Published: December 15, 1975
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