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Iwao Hosokawa
1989 Volume 58 Issue 4 Pages
1125-1127
Published: April 15, 1989
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It is a well-known but very puzzling fact that the probability density of spatial distribution of the vorticity magnitude in isotropic turbulence is nearly exponential. This fact is explained on the basis of a simple vortex model for 3D homogeneous turbulence.
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Hideo Sugama, Masahiro Wakatani
1989 Volume 58 Issue 4 Pages
1128-1130
Published: April 15, 1989
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Pressure-driven interchange instability of any mode number with the same helicity has the same limiting beta value as that by the Suydam criterion in the cylindrical plasma approximation. Growth rate of the Suydam mode gives an upper boundary of that of the low mode number interchange instability. It is possible that conventional numerical calculations using finite mesh sizes give a higher beta limit by the low mode number interchange instability than the Suydam limit because they fail to find sharply localized modes with small growth rates.
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Hidetsugu Kitatani, Takehiko Oguchi
1989 Volume 58 Issue 4 Pages
1131-1134
Published: April 15, 1989
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The three-dimensional ±
J Ising model on the simple cubic lattice is studied by means of the screw transfer matrix method for
L×
L×
N lattices (
L=2∼5;
N\simeq10
3). Studying the decay of the correlation functions, the value of the critical exponent η is found to be −0.26±0.03, assuming
Tsg⁄
J=1.2. The result is in good agreement with that obtained by the Monte Carlo method and high temperature series expansion method.
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Masaki Maeda, Tooru Atake, Yasutoshi Saito, Hikaru Terauchi
1989 Volume 58 Issue 4 Pages
1135-1136
Published: April 15, 1989
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Specific heats of betaine phosphate were measured in the temperature region from liquid helium temperature to room temperature. Two specific heat anomalies were found at 82.67 K and 87.11 K due to a new phase transition and the antiferroelectric phase transition, respectively. The sum of the two transition entropies was determined as 0.40 J K
−1 mol
−1.
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Migaku Oda, Tatsuya Ohguro, Naofumi Yamada, Masayuki Ido
1989 Volume 58 Issue 4 Pages
1137-1140
Published: April 15, 1989
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Temperature dependence of magnetic susceptibility χ and resistivity in (La
1−xSr
x)
2CuO
4 has been examined in a composition range of
x≤0.15. For
x\lesssim0.1, χ gradually decreases with lowering temperature, accompanied by a broad peak, while for
x>0.1 χ monotonically increases with decreasing temperature. Superconducting transition temperature
Tc is observed to be high in samples with
x\lesssim0.1, although
Tc is depressed with a steplike behavior below
x\simeq0.08.
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Nobuaki Miyakawa, Daisuke Shimada, Tadaharu Kido, Nobuo Tsuda
1989 Volume 58 Issue 4 Pages
1141-1144
Published: April 15, 1989
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Anisotropy in the energy gap of Bi2212 was investigated by using a point contact tunneling junction and it was noted that there was very little anisotropy. When a GaAs needle was contacted perpendicular to the
c-plane, at least two kinds of conductance curves were obtained, one with a gap of 42 meV and the other with a gap of 64 meV. In the latter, phonon structures extended to a higher voltage and a three-phonon process was observed similar to our multiphonon exchange model for superconductivity.
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Shunsuke Takano, Eiji Kita, Kiiti Siratori, Kay Kohn, Shigeyuki Kimura ...
1989 Volume 58 Issue 4 Pages
1145-1148
Published: April 15, 1989
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The structural change in YIG at 125 K is revealed by the observation of the first-order magnetoelectric effect. From the detailed experiments at 77 K with different field cooling conditions, it is concluded that the magnetic point symmetry of YIG below 125 K is triclinic-1.
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Kazuyuki Matsumoto, Takayuki Abe, Takeo Izuyama
1989 Volume 58 Issue 4 Pages
1149-1151
Published: April 15, 1989
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The exchange narrowing of the nuclear magnetic relaxation time
T1 of bcc
3He is investigated. It is found that multiple exchange models with two and three parameters may explain the
T1 data observed in the region 0.2<
T<0.8 K for
Vm=24.2 cm
3/mol. We investigate further the narrowing in hcp
3He. Based on the multiple exchange model with the exchange parameters
J1,
J1′,
J2, and
Ksq, we obtain a theoretical expression for
T1.
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Miki Wadati, Yasuhiko Yamada, Tetsuo Deguchi
1989 Volume 58 Issue 4 Pages
1153-1161
Published: April 15, 1989
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A formula for eigenvalues of the braid generator is derived from the Knizhnik-Zamolodchikov equation in conformal field theory. Through the formula, reduction relations are calculated. They agree with the results previously obtained in the study of new link polynomials. This establishes an explicit connection between knot theory based on exactly solvable models and conformal field theory.
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Yohtaro Ueno, Gang Sun, Ikuo Ono
1989 Volume 58 Issue 4 Pages
1162-1181
Published: April 15, 1989
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We develop an interface approach to bulk phase transitions and ordered states by using Monte Garlo simulations, and apply it to antiferromagnetic
q-state Potts models with
q=3∼6 on the simple cubic lattice. A stiffness exponent
a defined by
ΔF∼
La, where
ΔF is the interface free energy for a system of size
L, is introduced as a measure of the stiffness of the ordered phase against an external stress. Applying finite-size scaling to
ΔF and to the squared order parameter enable one to determine each of
Tc, ν, β and γ in order where
Tc is the critical temperature and the others are critical exponents. This approach also provides a means to study properties of the ordered state through
a and interface profiles. In the
q=3 and 4 models the estimated exponents ν, β, γ and
a indicate new universality classes. The
q=5 model shows a phase transition, while the
q=6 model does not. The
q=3∼5 models have non-integer values of a at low temperatures. The phase transitions in these models are confirmed to be due to entropy gains.
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Masakazu Ichiyanagi, Kunisuke Nisizima
1989 Volume 58 Issue 4 Pages
1182-1189
Published: April 15, 1989
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A general evolution criterion, applicable to transport processes such as the conduction of heat and mass diffusion, is obtained as a direct version of the Le Chatelier-Braun principle for stationary states. The present theory is not based on any radical departure from the conventional one. The generalized theory is made determinate by proposing the balance equations for extensive thermodynamic variables which will reflect the character of convective systems under the assumption of local equilibrium. As a consequence of the introduction of source terms in the balance equations, there appear additional terms in the expression of the local entropy production, which are bilinear in terms of the intensive variables and the sources. In the present paper, we show that we can construct a dissipation function for such general cases, in which the premises of the Glansdorff-Prigogine theory are accumulated. The new dissipation function permits us to formulate a generalized evolution criterion for convective systems.
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Nobuaki Tomita, Hiroshi Orihara, Yoshihiro Ishibashi
1989 Volume 58 Issue 4 Pages
1190-1198
Published: April 15, 1989
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Time evolution of domain patterns in a quenched ferroelectric triglycine sulphate (TGS) crystal is investigated in real time and in real space. The effect of applying an electric field after quenching is studied. The characteristic length, defined as a mean domain width, is found to obey the power law with respect to time. From the experimentally obtained time dependence of the area fraction of the domains with positive and negative polarization, it is found that this system behaves like one with a conserved order parameter in the studied time scale, though the order parameter in TGS is the polarization. For the system, to which the electric field is applied, it is found that the dynamical scaling law holds for the domain size distribution function.
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Yoshitaka Tanimura, Ryogo Kubo
1989 Volume 58 Issue 4 Pages
1199-1206
Published: April 15, 1989
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Two-time correlation functions of physical operators of a system interacting with a heat bath producing a Gaussian-Markoffian noise are treated with the use of Feynman-Vernon’s influence functional formalism. The Laplace transforms of correlation functions are shown to be expressed in terms of continued fractions of relevant hyperoperators. The result is valid to all orders of the system-bath interaction. In the limitation of motional narrowing, it reduces to those obtained in conventional methods.
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Hiromi Otsuka
1989 Volume 58 Issue 4 Pages
1207-1212
Published: April 15, 1989
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We propose a method for obtaining the average values of physical quantities at temperatures different from the assumed value from a simulation calculation of the constant temperature molecular dynamics (MD) with a fixed temperature. The method is developed on the basis of Nosé’s canonical MD. The present method is numerically tested in a simulation on a 13-atom Lennard-Jones cluster.
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Willem Overlaet, Masahiro Kimura, Shuichi Kinoshita, Takashi Kushida
1989 Volume 58 Issue 4 Pages
1213-1224
Published: April 15, 1989
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The spectrum of secondarily emitted light from iodine vapor excited by a single-mode Ar
+ ion laser has been measured in the forward scattering geometry with a resolution of 80 MHz. The observed spectrum has been found to consist of sharp and broad components. This result is shown to be reproduced fairly well by a Monte Carlo simulation of the molecular collision. The cross sections for the soft and hard velocity-changing collisions of an I
2 molecule in the excited state have been obtained as 230 Å
2 and 80 Å
2, respectively.
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Ahmed E. Radwan
1989 Volume 58 Issue 4 Pages
1225-1227
Published: April 15, 1989
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Instability of a gas cylinder in a moving infinite liquid under the action of capillary and inertia forces is discussed. The motion of the liquid has always a destabilizing influence, which increases the region of instability. But, the longitudinal wave number for the maximum instability does not change with the liquid velocity.
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Nobuaki Ikuta, Y\={u}hei Sugai
1989 Volume 58 Issue 4 Pages
1228-1247
Published: April 15, 1989
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Using the newly developed “flight time integral” method, we have carried out a rigorous analysis of the electron transport property in a model gas under the influence of electric and magnetic fields. As is well known, the electron energy distribution is not changed by addition of the magnetic field
B in parallel to the electric field
E, but is seriously changed when a crossed magnetic field is given above a critical value
Bc, where all the electron transport coefficients are diminished with
B. It is confirmed that the similarity law holds only when all the values of
E,
B and gas density
N are changed together, keeping
E⁄
N and
B⁄
N constant.
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Katsumichi Hoshino, Takumi Yamamoto, Hisato Kawashima, Toshihiko Yamau ...
1989 Volume 58 Issue 4 Pages
1248-1264
Published: April 15, 1989
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The gradient of the edge electron temperature during a tokamak H-mode and parameter dependences of the threshold peripheral electron temperature are measured by the
electron
cyclotron
emission (ECE). A steep gradient characterizes the H-mode and the threshold temperature is dependent on the plasma current. The second H-mode transition is observed, which is characterized by further depression of the intensity of deuterium line, and steeper gradient at the edge. A simple estimation using the measured gradient gives an improvement of the electron heat diffusivity at the pedestal. Some problems are discussed by comparing the measured results with the existing H-mode theories.
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Shiro Asano, Makoto Ihara, Masayuki Fukao
1989 Volume 58 Issue 4 Pages
1265-1272
Published: April 15, 1989
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A method to trap a high temperature and high density plasma from a coaxial gun in a mirror machine is described. The method is to inject plasma parallel to the axis from a coaxial gun located off the axis. The validity of the method is experimentally demonstrated with an MHD-stabilized axisymmetric mirror with an internal hoop. Density, electron and ion temperatures and their time behaviors were measured and it was made clear that a high density high temperature plasma was well trapped in the mirror by the parallel off-axis injection while the plasma was little trapped by on-axis injection. The plasma parameters obtained were also compared with those of a conventional titanium washer gun plasma. The causes to restrict the maximum ion temperature and of its quick decay are discussed.
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Tatsuo Watanabe, Yasuo Kanamori, Nobuo Yajima
1989 Volume 58 Issue 4 Pages
1273-1282
Published: April 15, 1989
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A stationary structure of a sheath around a negatively biased grid inserted in a homogeneous plasma and the associated effects on propagation characteristics of ion-acoustic waves are studied with a theory of collisionless plasma. The reductive perterbation method is applied to obtain the reflection coefficient of ion-acoustic waves from the grid. The results are shown to be in good agreement with the experiments by Nishida and Nagasawa.
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Junichi Yoshimura
1989 Volume 58 Issue 4 Pages
1283-1295
Published: April 15, 1989
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Interference fringes in X-ray diffraction must be a projected figure thrown to the wave-traveling direction, due to the property of the wave field that
ΔK=const. along the wave path and
ΔK⊥\bar
K(
ΔK=
K′−
K and (
Remark: Graphics omitted.)),
K and
K′ being the wave vectors of interfering waves in vacuum). The second property comes from the condition |
K|=|
K′|. The question of whether moiré fringes have this projective property was examined experimentally. Moiré fringes were observed from a monolithic Si bicrystal by X-ray topography. Experiments have shown that the directions and positions of moiré fringes vary with the shift of the observation point along the wave path in oscillatory manners, and thus the moiré fringes are not exactly the projected figure. This fact indicates that the first or both of the conditions,
ΔK=const. and
ΔK⊥\bar
K, do not apparently hold in the moiré-fringe interference.
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Kazuo Nakanishi
1989 Volume 58 Issue 4 Pages
1296-1306
Published: April 15, 1989
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Mean field calculations are made to study the effect of nonlinear terms with respect to the magnetization in the axial next-nearest neighbor Ising (ANNNI) model. The phase diagrams are calculated in both zero and nonzero magnetic fields, in which a large number of high-order commensurate phases is found. It is shown that the nonlinear effect makes the ordered phase stable at higher temperatures and larger fields. Partially disordered states which contain paramagnetic sites are also obtained, resulting from the nonlinear effect as well as the competition between the intralayer coupling and the entropy effect. In this connection, the theory is compared with the complex magnetic phase diagram of CeSb.
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Ryuzo Abe
1989 Volume 58 Issue 4 Pages
1307-1311
Published: April 15, 1989
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By extension of a previous treatment, the principle of corresponding state for fluid metals is derived. The ion is regarded as a hard sphere with a core radius
b. Dimensional analysis of the Schrödinger equation for an electron system leads to the result that four independent parameters appear to characterize the thermodynamic properties of the system. By a choice of suitable parameters, some relations between critical quantities are studied for a series of alkali metals. Also, a possible dependence of the critical compressibility factor and of the reduced equation of state on
Z (valence of ion) is discussed.
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Ippei Doi
1989 Volume 58 Issue 4 Pages
1312-1319
Published: April 15, 1989
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Based on the quantum lattice gas model, the superfluid transition temperature
Tc is calculated for
4He atoms in the model substrate of zeolite. When the density in void cages and that in pores is different,
Tc is strongly reduced compared with the case that the density is homogeneous. In particular, if a pore is longer than a certain length, the superfluidity completely disappears under any density. This makes a contrast with the case of the homogeneous density where
Tc remains finite for each pore length. We also give a general discussion on the competition between the superfluid transition and the solid-liquid (or liquid-gas) transition of bose particles in zeolite.
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Katsumi Yoshino, Yasuhisa Manda, Keiji Sawada, Shigenori Morita, Hiroy ...
1989 Volume 58 Issue 4 Pages
1320-1324
Published: April 15, 1989
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Poly(3,4-dialkylthiophene) films prepared by both electrochemical and chemical methods utilizing FeCl
3 as catalyst exhibit much larger band gap compared with non-substituted and 3-substituted polythiophene films. Poly(3,4-dialkylthiophene)s with long alkyl chains are soluble in several solvent. However, thermochromism has not been found contrary to poly(3-alkylthiophene), which are explained in terms of large torsion angle between neighbouring thiophene rings due to the steric hindrance by bulky alkyl group. Poly(3,4-dimethylthiophene) with large band gap also demonstrates drastic spectral, electron spin resonance (ESR) and conductivity changes upon doping due to an insulator-metal transition.
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Shuichi Iwabuchi, Yosuke Nagaoka
1989 Volume 58 Issue 4 Pages
1325-1333
Published: April 15, 1989
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Effect of intersubband impurity scattering on the Anderson localization is studied in the weakly localized regime of two dimensional electron systems. It is shown that it changes not only the prefactor of the quantum correction of conductivity, but also the diffusion constant, depending on the ratio of the intersubband scattering time to the inelastic scattering time. The crossover behavior in magnetoconductivity from one-subband occupation to two-subband occupation is also studied. Since it varies depending on various scattering times, details of scattering processes can be determined for an arbitrary electron density by fitting experimental observations to theoretical expressions. Experimental determination of the inelastic scattering time without considering this effect leads to an incorrect estimation.
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Nobuhisa Fujima, Tsuyoshi Yamaguchi
1989 Volume 58 Issue 4 Pages
1334-1346
Published: April 15, 1989
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Electronic states of icosahedral (Ih) clusters Al
13, Al
12, Cu
13 and Cu
12 were calculated by the DV–Xα method which took into account of many-electron effects. The valence 3
d orbitals of Ih–Cu
13 cluster are localized within atom and isolated from the valence 4
s and 4
p orbitals extended over the whole cluster. The characteristic feature of the states of
s and
p valence electrons of Ih–Al
13 and Cu
13 clusters well corresponds to that of one-electron picture i.e. the shell model of the 3-dimensional isotropic harmonic oscillator potential. Electronic states of valence levels of Ih–Al
12 and Ih–Cu
12 clusters which have no central atom fairly well correspond to those of a combined potential of the harmonic oscillator and a 3-dimensional Gaussian potential barrier at the center of the cluster.
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Yasuhiro Hatsugai, Masatoshi Imada, Naoto Nagaosa
1989 Volume 58 Issue 4 Pages
1347-1371
Published: April 15, 1989
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A coupled spin-fermion system is investigated as a model of high-
Tc superconductivity. By the exact diagonalization technique, the binding energy of two fermions and several correlation functions in the ground state are calculated to study possible pairings of holes in orbitals of
pπ,
pσ,
d3z2−r2 etc. The bound states of fermions are suggested in two regions in the parameter space. In the small transfer region, it is caused by local defects induced in the antiferromagnet at the fermion sites. The larger transfer region is characterized by the relatively extended disturbance of the antiferromagnetic correlation of the substrate spins, where the fermion forms singlet-like cloud around it. The latter is a characteristic feature of the antiferromagnetic fermion-spin coupling. The relevance of the latter region to high-
Tc superconductivity is discussed. The possibilities of bound states of fermions in Kondo lattices are also investigated.
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Mitsuru Morita, Kazuhiko Yamaya
1989 Volume 58 Issue 4 Pages
1372-1376
Published: April 15, 1989
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To make clear the mechanism of “the giant resistivity anomaly” appearing in the superconducting transition region of TaSe
3, the experimental conditions are re-examined. It was found that the anomaly is not intrinsic but is induced by a coupling between the non-linear current-voltage characteristics of TaSe
3 and the high-frequency noise generated by instruments. From the measurement of the superconducting critical current, it was concluded that the superconductivity of TaSe
3 is not of bulk nature but filamentary.
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Ryusuke Ikeda, Tetsuo Ohmi, Toshihiko Tsuneto
1989 Volume 58 Issue 4 Pages
1377-1386
Published: April 15, 1989
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We attempt to explain the broad resistive transition observed in high-temperature superconductors under an applied magnetic field by a renormalized theory of the order parameter fluctuations using a model of superconductors with layered structures. The results are compared with single-crystal resistivity data. They are in good agreement, at least in the higher temperature side of the resistive transition, where the theory is expected to be valid.
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Kazuo Hida
1989 Volume 58 Issue 4 Pages
1387-1393
Published: April 15, 1989
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A model of the high-
Tc oxide superconductor based on the antiferromagnetic spin wave exchange is investigated. It is assumed that the holes, which are the superconductive carriers, are mainly doped into the p
π orbital of the O atoms on the CuO plane. Cu spins are assumed to be localized and to be in the almost antiferromagnetic state. In this case, the O holes can form Copper pairs exchanging the spin wave of the Cu spin system. The transition temperature is calculated taking into account the lifetime of the spin wave and the retardation effect. The carrier density dependence of the transition temperature is discussed. The structure of the energy gap and the real space pair-wave function is presented. The Cooper pair is shown to have d-like symmetry.
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Hiroyuki Mori
1989 Volume 58 Issue 4 Pages
1394-1402
Published: April 15, 1989
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We investigate superconductivity in a two-dimensional square lattice characterized by both an on-site attractive interaction (−
V1) of the
BCS type and an inter-site attractive interaction (−
V2). We evaluate the phase diagram in the (
V1,
V2,
T) space, which shows that there appear three kinds of superconducting states, i.e. a pure
s-state, a pure
d-state and a mixed state, depending on the values of
V1,
V2, and
T. For some appropriate values of
V1 and
V2, two types of transitions take place on the reduction of temperature; from a normal state to a pure state and then from a pure state to a mixed state. We calculate several physical quantities in order to study their behaviors at these transition points. Implication of the present theory is discussed in relation with high-
Tc superconductivity.
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Takehiko Oguchi, Hidetsugu Kitatani
1989 Volume 58 Issue 4 Pages
1403-1415
Published: April 15, 1989
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The theory of the resonating valence bond (RVB) for the antiferromagnetic Heisenberg model of spin 1/2 proposed by Anderson is generalized by taking account of singlet bonds connecting distant spins, and is solved exactly for the finite lattice. It is shown that the RVB wave function is
Stot (total spin quantum number)=0, and that replacing a part of singlet bonds by triplet bonds, eigenfunctions with
Stot=1, 2, … can be constructed. These are the new representation of eigenfunctions of the Heisenberg Hamiltonian.
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Hideki Yoshizawa, Setsuo Mitsuda, Hiroko Aruga, Atsuko Ito
1989 Volume 58 Issue 4 Pages
1416-1426
Published: April 15, 1989
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Neutron scattering demonstrates the clear reentrant spin-glass (SG) transition, for the first time, in the Ising system Fe
xMn
1−xTiO
3 for
x=0.33, 0.38, 0.60, and 0.65. The samples with
x=0.41, 0.50 and 0.55 exhibit paramagnetic to SG behavior upon lowering the temperature. The results confirm the SG and reentrant SG transitions which were suggested from the previous bulk susceptibility measurements by Ito
et al. The reentrant SG phase is shown to be actually a mixed phase where the antiferromagnetic long range order coexists with the SG ordering. The behavior of the diffuse intensity as well as the inverse correlation length κ as a function of an Fe ion concentration
x strongly suggests that there exists a phase boundary between the mixed phase and the pure SG phase. Thus the phase below the AT line in an Ising SG system should be strictly distinguished from the pure SG phase. By comparing the data of the
x=0.58 sample to that of the
x=0.57 sample, this phase boundary is parallel to the temperature axis within the accuracy of 0.5% of the Fe concentration. The topology of the Ising SG phase diagram is briefly discussed by contrast to that of the Sherrington-Kirkpatrick model.
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Norio Kawakami, Tatsuya Usuki, Ayao Okiji
1989 Volume 58 Issue 4 Pages
1427-1432
Published: April 15, 1989
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The magnetization curve for the Ce Kondo system is investigated with the use of the exact solution of the Coqblin-Schrieffer model at zero temperature. Characteristic properties caused by the crystal-field effects are discussed with a simple level scheme for the hexagonal field. The obtained results are quantitatively compared with experimental findings for the heavy electron compounds CeAl
3 and CeCu
2Si
2 with rather good agreement.
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Midori Tanaka, Hiroko Iwasaki, Kiiti Siratori, Isamu Shindo
1989 Volume 58 Issue 4 Pages
1433-1440
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Mössbauer spectra of
57Fe in a single-crystal YbFe
2O
4, an antiferromagnetic Ising spin system on a triangular lattice, were measured below the Neel temperature,
TN. Outermost groups of absorption spectra, those due to Fe ions in a 3+-like state, were investigated extensively as a function of the external magnetic field during measurement (
Hmeas) as well as that during cooling (
Hcool) of the specimen through
TN. It is concluded that there are three kinds of Fe
[3+] ions of equal number, the spins of two of which are parallel to each other and antiparallel to the other. The effective field at the nuclei of the majority Fe
[3+] spin is increased by
Hmeas. Formation of short-range ordering of Fe ions with different valences is suggested, though the details are not clear at present.
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Jun Takeda, Takenari Goto, Makoto Tomita, Masahiro Matsuoka
1989 Volume 58 Issue 4 Pages
1441-1445
Published: April 15, 1989
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A new luminescence band has been found in the temperature range from 40 to 80 K under high-density excitation of 2H-PbI
2. The decay time of this luminescence at 58 K is about 400 ps, which is twice as large as that due to the excitonic molecule, and both the Stokes shift and the half-width are about 0.01 eV. These experimental facts suggest that the new luminescence comes from radiative annihilation of the self-trapped excitonic molecule leaving the exciton in the distorted lattice.
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Raphael Ruppin
1989 Volume 58 Issue 4 Pages
1446-1451
Published: April 15, 1989
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The absorption cross section of a system of two spheres is derived by an analytic method based on the separability of the Laplace equation in bispherical coordinates. The method is applicable in the non-retarded limit, i.e., for sphere radius small in comparison with the wavelength of the impinging electromagnetic radiation. The evolvement of the absorption spectrum with decreasing distance between the spheres is demonstrated by numerical calculations. The implications on the interpretation of experimental infrared absorption spectra of small crystallites are discussed.
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Takeo Jo
1989 Volume 58 Issue 4 Pages
1452-1463
Published: April 15, 1989
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The effect of valence mixing on multiplet structures in the Ce 4
d X-ray absorption spectra for metallic Ce compounds such as CeRh
3 and insulators CeO
2 and CeF
4 is discussed on the basis of the impurity Anderson model combined with the electron-electron (or hole) interactions described by the Slater integrals and the spin-orbit interactions. A similarity in the spectrum for a prethreshold region between metallic mixed valent compounds such as CeRh
3 with the number of 4
f electrons
nf∼0.8 and trivalent compounds (
nf∼1) and a dissimilarity between CeRh
3 and the insulators CeO
2 (
nf∼0.5) and CeF
4 (
nf∼0.3) are explained consistently with an interpretation for their 3
d core level spectra. The deviation from the multiplet structure typical of integral valence system is shown to be caused by a strong interference between the 4
d104
f0→4
d94
f1 and 4
d104
f1v→4
d94
f2v photoexcitations which is derived from the hybridization between the 4
f and conduction (or valence) band states.
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Yoshinori Hayashi, Hideyuki Nakagawa, Hiroaki Matsumoto
1989 Volume 58 Issue 4 Pages
1464-1473
Published: April 15, 1989
Released on J-STAGE: May 29, 2007
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Emission intensities, lifetimes and their temperature dependence of the UV-emission in the CdI
2:Br mixed crystals were investigated from 1.7 to 50 K by varying the Br
− concentration and the excitation energy. The UV-emission is observed in the region between 3.30 and 3.45 eV and diminishes as increasing the concentration of CdBr
2. The UV-emission decays with three exponential components: τ
S=83 μs, τ
M=24 μs and τ
F=2.3 μs at 1.7 K. It has been proved that the initial state of the τ
S-component and that of the τ
M- and τ
F-components are quite distinct from each other. In order to explain the present experimental results three exciton relaxation processes into the UV-states are proposed, that is, the tunneling and the thermal activation processes from the bottom of the indirect free exciton band and the direct process from the upper states of excitons.
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Yoshitaka Yamamoto, Takahiro Yamaguchi, Kuninosuke Imaeda
1989 Volume 58 Issue 4 Pages
1474-1481
Published: April 15, 1989
Released on J-STAGE: June 01, 2007
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Responding to an external periodic force, the oscillation mode of the Oregonator shows a hysteresis phenomenon and a relaxation phenomenon according as the final value of the amplitude is inside or outside of the bistable region where the amplitude of the external periodic force is varied with time while the frequency is kept constant. In the outside of the bistable region and in the vicinity of the transition points, we observed relaxation phenomena and obtained the critical exponent in the relation between the relaxation time and the difference of the control parameter from the critical point.
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Yoshihisa Mori, Yuichi Akahama, Mototada Kobayashi, Haruki Kawamura, K ...
1989 Volume 58 Issue 4 Pages
1482-1483
Published: April 15, 1989
Released on J-STAGE: May 29, 2007
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Shin’ichi Takeda, Shigeru Tamaki
1989 Volume 58 Issue 4 Pages
1484-1485
Published: April 15, 1989
Released on J-STAGE: May 29, 2007
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Tetsuhiko Tomiki, Tomoyoshi Futemma, Hiroo Kato, Tsuneaki Miyahara, Yo ...
1989 Volume 58 Issue 4 Pages
1486-1487
Published: April 15, 1989
Released on J-STAGE: June 01, 2007
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Keiichi Edamatsu, Takao Nanba, Mikihiko Ikezawa
1989 Volume 58 Issue 4 Pages
1488
Published: April 15, 1989
Released on J-STAGE: May 29, 2007
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