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Kiyoshi Murakawa
1962 Volume 17 Issue 6 Pages
891-896
Published: June 05, 1962
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The shielding correction
Δ defined by
Q=(1+
Δ)
Q′ (
Q=true quadrupole moment;
Q′=apparent quadrupole moment obtained by spectroscopic means neglecting the shielding effect) was investigated in the cases of the state 5
d46
s of Ta I and 5
d66
s6
p of Os
189 I. In these cases the correction
Δ for the group 5
d46
s or 5
d66
s was found to be of the order of 9±5; namely the shielding effect predominates over the antishielding effect. It is highly probable that
Δ is around zero in the state 5
d6 of Os I. The quadrupole moment of Os
189 is 0.8±0.2 barn. The hyperfine structure due to Os
187 was also studied, and μ(187)=+0.0656±0.0006 nm, was obtained.
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Kunio Takamatsu
1962 Volume 17 Issue 6 Pages
896-906
Published: June 05, 1962
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The angular distributions of the emitted alpha particles from the (
d, α) reactions on F
19, Ne
20, P
31 and S
32 leading to the ground states and several excited states of the residual nuclei have been measured at an incident deuteron energy of 14.7 Mev. The emitted alpha particles were detected with a solid state detector of a silicon p-n junction.
The alpha particle groups, α
0 of the ground state transitions for all targets and the alpha particle groups of several excited state transitions for F
19 and S
32 show pronounced peaks at forward angles and oscillatory behaviors in the angular distributions, which were compared, and were in good agreement, with the theory of the two nucleon pickup process.
The angular distributions of other alpha particle groups for excited state transitions show nearly symmetrical behaviors about 90° and the cross sections of them are smaller by about a factor of 2∼5 than those of α
0. These facts suggest that these reactions occur through different process, and are consistent with the level structures of residual nuclei predicted from the shell model.
The mass number dependence of the integrated cross sections for the ground state transitions was obtained. The values of the cross sections are proportional to the inverse cubes of mass number
A and the values of the cross sections for even-even nuclei are larger by about a factor of 3 than those for odd-odd and odd nuclei, in the mass region 14\lesssim
A\lesssim 32.
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Soji Kono
1962 Volume 17 Issue 6 Pages
907-914
Published: June 05, 1962
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The decay of Ga
68 (68 min) has been investigated with beta- and gamma-ray scintillation spectrometers. Two beta-ray components with endpoint energies of 1.95±0.03 MeV, and 0.88±0.05 MeV are observed. Gamma-rays of 0.80±0.02, 1.08±0.01, 1.24±0.02 and 1.88±0.01 MeV are confirmed. Angular correlation of the 1.08–0.80 MeV gamma-ray cascade in Zn
68 have been measured. The Legendre polynomial expansion coefficients are determined to be
A2=−0.237±0.056 and
A4=0.39±0.062. The measured correlation establishes the spin sequence to be 2–2–0, with a quadrupole-dipole mixing ratio δ of −(4
−2+3) for the 0.80 MeV gamma-ray. The results of the angular correlation work together with the allowed nature (log
ft=5.7) of the electron capture decay to the 1.88 MeV level fix the spin and parity of this level to be 2+. The results are consistent with the systematics given by Sakai for low excited of even states of even-even nuclei.
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Takuji Yanabu, Sukeaki Yamashita, Teruo Nakamura, Kunio Takamatsu, Aki ...
1962 Volume 17 Issue 6 Pages
914-920
Published: June 05, 1962
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The angular distributions have been measured for the eight groups of alpha particles leading to the ground state and the excited states of Mg
25 from the reaction Al
27(
d, α)Mg
25 with 14.7 MeV deuterons, by using a semiconductor detector of
p-
n junction. The differential cross-sections of the reactions leading to the single levels of Mg
25 are compared with a formula obtained from the two-nucleon pick-up theory. The experimental angular distribution for each alpha group with a comparatively large cross-section is in agreement, at least in forward angle, with the theoretical curve. The alpha group leading to the 3.40 MeV level of Mg
25 is considered to come from the transition to the 9⁄2+ state rather than to the 3⁄2− state. The total cross-sections for the levels of Mg
25 corresponding to the same
K-band 5⁄2+ as that of the ground state of Al
27 are larger than the others.
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Yoshiichi Fukuda, Kazuhiko Yoshida
1962 Volume 17 Issue 6 Pages
920-923
Published: June 05, 1962
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Using the moment method, the frequency spectrum of lattice with short range order is calculated. It is shown that the spectrum of the lattice comes to resemble the spectrum of the ordered lattice as the short range order increases.
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Hiroo Toyoda, Masayuki Itakura
1962 Volume 17 Issue 6 Pages
924-931
Published: June 05, 1962
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The effect of electrode materials and atmospheres on the polarization reversal and the electrical conduction of barium titanate single crystals were investigated. It was revealed From d. c. conduction measurements that evaporated indium and tellurium metals give an ohmic and a blocking contacts, respectively. It was found that the switching rate under the application of sinusoidal field is primarily determined by the anode substance and that the indium electrode markedly slows down the rate. The polarization reversal of the crystals with evaporated gold electrodes is affected considerably by atmosphere. The switching rate was decreased by evacuation and increased by the adsorption of polar molecules. The switching behavior was determined by the atmosphere in contact with anode. The condition to bring about a sharp switching required at least one blocking contact so biased that the carriers were easy to flow across it. The mechanism is discussed.
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Kazuo Kanematsu, K\={o} Yasukochi, Tetuo Ohoyama
1962 Volume 17 Issue 6 Pages
932-936
Published: June 05, 1962
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The susceptibilities of Co
1.67Ge and Ni
1.67Ge are nearly independent of temperature, and the values are 4.9×10
−6 and 0.4×10
−6 emu/g respectively. From the magnetic measurement on a series of alloys of (Co, Ni)
1.67Ge, it is concluded that these alloys are of Pauli paramagnetism. The density of states is calculated as a function of energy, and then the effective mass ratio is estimated on the basis of the free electron theory. The ratio
m*⁄
m is about 28 for cobalt rich side, and 5 for nickel rich side. Therefore the magnetism of Co
1.67Ge and Ni
1.67Ge may be ascribed to the Pauli paramagnetism of 3
d holes and 4
s electrons respectively. These conclusion is consistent with a theory previously proposed.
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Rinjiro Ando
1962 Volume 17 Issue 6 Pages
937-940
Published: June 05, 1962
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Dielectric constant, thermal expansion coefficent,
dc resistivity, and pyroelectric current of KLiSO
4 were measured in the temperature range covering its transition point. The former three quantities revealed anomalies at the transition point and the temperature hysteresis of about 10°C was observed. The D-E curve showed no anomaly and the reversion of the pyroelectric current by the
dc poling was not observed. It is concluded that the crystal is polar but not ferroelectric.
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Hideo Nukushina
1962 Volume 17 Issue 6 Pages
941-949
Published: June 05, 1962
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The space-charge layer width and the junction capacitance of a hyper-abrupt
p-
n junction were studied, especially on the characteristics of temperature-dependence. The solution of Shockley’s equation in space-charge case gives a fairly good approximation of the characteristics of such a junction. The temperature dependence of the space-charge layer width can be explained mainly by the change in the built-in barrier voltage. However, there still remains a tendency that, at higher temperature, the space-charge layer width is narrower than that of the expected magnitude.
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Kin-ichi N\={o}ga
1962 Volume 17 Issue 6 Pages
950-961
Published: June 05, 1962
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The field emission microscope has been used to investigate the state of adsorption of barium oxide molecules deposited on tungsten by evaporation. Precautions are taken so as to keep the tube pressure at ultra high vacuum. Pulse method is adopted to protect the state of adsorption from changing with steady application of intense fields.
Surface migration of adsorbed molecules over the entire surface is pronounced only above 700°C and its activation energy is about 4.6 eV.
Work function decreases very rapidly for the first 0.15 layer with the rate which can be explained quantitatively by considering the adsorbed molecules as oriented dipoles. The mean dipole moment of an adsorbed molecule is estimated to be (13.5±8.1)×10
−18 esu. Crystallites of barium oxide are formed when covering factor amounts to about unity.
Chemical reaction takes place between barium oxide and tungsten for temperatures above 800°C and the reaction product persists stably unless temperature is raised above 1000°C. The activation energy of the reaction is about 3.3eV
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Eiji Nakamura
1962 Volume 17 Issue 6 Pages
961-966
Published: June 05, 1962
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Dielectric constants and loss tangents of NaNO
2 and (Glycine)
3·H
2SO
4(TGS) single crystals have been measured at 3.3 kMc/s by the resonant cavity method from room temperature to 200°C for NaNO
2 and to 80°C for TGS. Dielectric constants measured along the
b-axes of the both crystals at 3.3 kMc/s are smaller than those at 1 Mc/s. No dielectric dispersion has been observed along the
a- and
c-axes of NaNO
2. Dielectric constants along these axes increase monotonically with temperature. The mechanisms of the dielectric dispersion of the both crystals are discussed in connection with their spectroscopic properties and crystal structures.
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Yukuo Kataoka
1962 Volume 17 Issue 6 Pages
967-969
Published: June 05, 1962
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Silicon films have been formed by the method of vacuum evaporation. The nature of the films has been observed by the studies of the effect of heat-treatment on resistivity, Hall mobility and X-ray diffraction.
Silicon was deposited on fused quartz substrates held at a certain temperature between 950°C and 1050°C. The films were generally subjected to heat-treatment after the deposition.
The films as deposited were generally
p-type, but the films made with the heat-treatment were converted to
n-type.
This tendency was ascribed to the boundary effects of crystallized particles or aggregations in the layer.
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Hajimu Kawamura, Masakazu Fukai, Yoshikazu Hayashi
1962 Volume 17 Issue 6 Pages
970-974
Published: June 05, 1962
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The experiment on cyclotron resonance of electrons in nearly intrinsic
n-type germanium with donor concentration of 7×10
12 cm
−3 was made at 1.6°K, making use of 6 mm microwave. The line shape as well as line width was measured as a function of power of microwave. For relatively high power (more than ten microwatts) the line width increases as (
P⁄
m*)
1⁄2,5, where
P is the microwave power and
m* is the mass along the direction of microwave electric field. The line shape is like Gaussian for higher power, while for low power it is Lorentzian. These facts were reasonably interpreted in term of rise of effective electron temperature due to the microwave absorption.
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Ryogo Kubo
1962 Volume 17 Issue 6 Pages
975-986
Published: June 05, 1962
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The level spacing of quantized electronic states becomes fairly large in very fine particles. For instance, it will be comparable to
kT at
T=1°K if the linear dimension of a particle is 50 Å or so. Thermal properties may show considerable deviations from the normal bulk values for such fine particles. The heat capacity will be reduced to about two-thirds and the paramagnetic susceptibility may be enhanced. Even more important effects are expected for relaxation processes. They are discussed briefly, but more detailed treatments will be given in a forth-coming paper.
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Yutaka Toyozawa
1962 Volume 17 Issue 6 Pages
986-1004
Published: June 05, 1962
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The co-operative effect of electron correlation and random lattice in the impurity conduction of semiconductors is investigated in terms of the Green’s function with in the frame-work of Hartree-Fock approximation. There appear magnetic states embedded in the metallic impurity band, being located at those impurity sites which are relatively isolated from other sites. The fraction of these magnetic sites is estimated to be of the order of ten percents, being a decreasing function of impurity concentration. The magnetic moment of the localized spin is calculated with a method which is different from the conventional one. Treating the localized spins as collective modes which act upon the individual electrons of the impurity band as potential fluctuation (in space and in time), we have calculated the effect of magnetic field or spin ordering on the electrical resistivity.
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Akira Yanase
1962 Volume 17 Issue 6 Pages
1005-1011
Published: June 05, 1962
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The time decrease of the magnetic permeability after demagnetization, so called disaccommodation, was observed for Ni–Zn ferrite, which had various degrees of oxidation. The effect of the existence of Fe
2+ ion in disaccommodation was detected. Fe
2+ facilitates the diffusion of cation and makes the disaccommodation rapid. Moreover, it was concluded that the induced anisotropy caused by the preferential occupation of cation vacancies is large enough to explain the disaccommodation in ferrite. The existence of some difference in diffusion rates among the constituent cations is necessary to explain the disaccommodation in ferrite.
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Kazuo Ôno, Atsuko Ito
1962 Volume 17 Issue 6 Pages
1012-1017
Published: June 05, 1962
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Mössbauer absorption by Fe
57 in α-Fe
2O
3 has been measured as a function of temperature from 100°K to 1050°K. In the hyperfine spectra, a steep change of the energy shift ε due to quadrupole interaction was found at about 260°K. The ratio of ε at 100°K to that at 300°K is −2.0±0.4. This value corresponds to the ratio of (3cos
2θ−1) below and above the transition temperature, if we assume that the direction of the principal axis of the electric field gradient at the iron nucleus is parallel to the
c axis.
A careful observation of the shape of the absorption line near the transition temperature showed that each line consisted of doublet respectively. This fact reveals that the transition temperature of α-Fe
2O
3 used in the present experiment varies locally from 220°K to 270°K. The value of
e2qQ obtained at about 260°K is (+0.084±0.008) cm/sec=(+9.7±,0.9) Mc/sec. Although there were fairly large errors in the obtained values of
e2qQ, thefild gradient seemed to increase slowly with temperature from 100°K to 700°K. Theabrupt increse of the field gradient was found near the Néel temperature. The observed temperature dependence of the internal magnetic field was fairly consistent with the molecular field theory for
S=5⁄2.
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Shunji Shirai, Yoshiichi Fukuda
1962 Volume 17 Issue 6 Pages
1018-1021
Published: June 05, 1962
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Using a model of an oriented f.c.c. metal deposited on the (001) plane of some f.c.c. metal, the conditions under which the (001) or (111) oriented overgrowth takes place are studied theoretically in terms of the forces due to the deposit and substrate atoms. The forces are assumed to be of the Lennard-Jones type. The theoretical result is in a fairly good agreement with the experimental one.
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Masao Kuriyama, Sukeaki Hosoya
1962 Volume 17 Issue 6 Pages
1022-1029
Published: June 05, 1962
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The atomic scattering factors of manganese and oxygen atoms in manganous oxide (MnO) were determined by measuring the integrated x-ray intensities of reflections from powder sample at room temperature. The intensities measured on a relative scale for five differently colored samples within an experimental error of ±0.4 to 4% were transformed to the absolute values by experimental scaling factors. The atomic scattering factors obtained were compared with those calculated by Watson and Freeman and by Suzuki and proved that the atoms were in the state of divalent ions. The tabulated anomalous dispersion terms were found to be reliable for Cu and Cr Kα radiations.
The effect of non-spherical charge distributions was discussed by a comparison between the experimental and the theoretical factors.
The lattice constant at room temperature was determined to be 4.444±0.001 A and thermal expansion coefficient above the Néel point, 1.1×10
−5 deg
−1. The root mean square amplitudes of thermal vibration were determined to be 0.12±0.03 A (
BMn=0.38 A
2) and 0.13±0.03 A (
Bo=0.45 A
2), respectively fir Mn and O ions.
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Sadae Yamaguchi, Denjiro Watanabe, Shiro Ogawa
1962 Volume 17 Issue 6 Pages
1030-1041
Published: June 05, 1962
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It has been confirmed by electron diffraction that anti-phase domains in Cu
3Au giving rise to diffuse superlattice reflections grow up during isothermal annealing below the transition temperature of order-disorder, evaporated films of nearly stoichiometric compositions being used. This fact means that anti-phase domains in Cu
3Au are not in an equilibrium state unlike the so-called periodic anti-phase structure.
Electron-microscopic images of domain boundaries of alloy films with 26 atomic per cent gold have been observed. These images also confirm the isothermal growth of domains. The irregular configuration of domain boundaries as observed by Fisher and Marcinkowski in electropolished specimens of Cu
3Au has been confirmed also in the evaporated films. It is concluded, however, that some correction should be made on the domain distribution of Cu
3Au suggested by these authors, on the basis of dark field images of electron micrographs formed by different kinds of superlattice reflection in the present study. The correct distribution is that in which the occupation of nearest neighbor positions by gold atoms is avoided as far as possible.
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Kazutake Kohra, Mitsuru Yoshimatsu
1962 Volume 17 Issue 6 Pages
1041-1052
Published: June 05, 1962
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Lattice defects in silicon single crystals are observed using Lang’s technique of X-ray diffraction microscopy. Lattice defects such as dislocations and two-dimensionally extended defects are observed only on one side of a twin boundary which is normal to the growth axis 〈111〉. Two-dimensional defect is concluded to be due to stacking fault from the study of the disappearance condition of the image with reflections. Fringe patterns due to stacking fualt is compared with the one due to a twinplane. The effect of heat-treatment on stacking faults are studied.
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Kanefusa Gotoh
1962 Volume 17 Issue 6 Pages
1053-1061
Published: June 05, 1962
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The present paper deals with the magnetohydrodynamic stability of laminar viscous flow between two rotating concentric circular cylinders in the presence of a circular magnetic field. Assuming that the difference between the radii of the inner and the outer cylinders is small compared with their arithmetic mean, the condition for the onset of instability is obtained. It is also found that in a special case when 4πνμσ=1, a simple relationship exists between the eigenvalues in magnetic and non-magnetic cases for arbitrary values of the amplification factor.
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T. Satyavati, P. Jayarama Reddy, S. V. Subrahmanyam
1962 Volume 17 Issue 6 Pages
1061-1064
Published: June 05, 1962
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Ultrasonic velocity and adiabatic compressibility have been studied as a function of composition for the systems: NaNO
3–Sr(NO
3)
2–H
2O; KNO
3Sr(NO
3)
2–H
2O, KCl–NaCl–H
2O; Pb(NO
3)
2–Sr(NO
3)
2–H
2O; KNO
3–Pb(NO
3)
2–H
2O, NaNO
3–Pb(NO
3)
2–H
2O; CdCl
2–KCl–H
2O; ZnCl
2–KCl–H
2O; CdBr
2–KBr–H
2O; ZnBr
2–KBr–H
2O; CdI
2–KI–H
2O; ZnI
2–KI–H
2O; CdCl
2–ZnCl
2–H
2O and CdBr
2–ZnBr
2–H
2O. The first six systems containing simple electrolytes like NaCl, KCl and NaNO
3 showed ideal behaviour i.e. linear variation of the compressibility and velocity. Solutions of cadmium halides and zinc halides in aqueous solutions of potassium halides are characterised by positive excess compressibility at a mole fraction of 0.666 of the potassium halide. This behaviour has been explained as due to the formation of complex ions of the type ZnX
4−− and CdX
4−−.
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Kunisuke Asayama, Junkichi Itoh
1962 Volume 17 Issue 6 Pages
1065
Published: June 05, 1962
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Shunsuke Kobayashi, Masaharu Aoki
1962 Volume 17 Issue 6 Pages
1066-1067
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Kazuo Kawabe
1962 Volume 17 Issue 6 Pages
1067
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Shigeru Waku
1962 Volume 17 Issue 6 Pages
1068-1069
Published: June 05, 1962
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Hiroshi Ohkura, Sei-ichi Nagata
1962 Volume 17 Issue 6 Pages
1069-1070
Published: June 05, 1962
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Takasi Ono, Teizo Takahama, Taizo Irie
1962 Volume 17 Issue 6 Pages
1070-1071
Published: June 05, 1962
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Hiroshi Yasuoka, Akira Hirai, Motohiro Matsuura, Tsuneo Hashi
1962 Volume 17 Issue 6 Pages
1071-1072
Published: June 05, 1962
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Keizô Aoyagi, Makoto Sugihara
1962 Volume 17 Issue 6 Pages
1072-1073
Published: June 05, 1962
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Shin-ichi Matsuoka, Shuzo Hattori
1962 Volume 17 Issue 6 Pages
1073-1074
Published: June 05, 1962
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Shozo Ino, Denjiro Watanabe, Shiro Ogawa
1962 Volume 17 Issue 6 Pages
1074-1075
Published: June 05, 1962
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Shigeko Miyamoto, Shin-ichi Nakashima, Hiroyuki Mizuno
1962 Volume 17 Issue 6 Pages
1076
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Hideo Suzuki
1962 Volume 17 Issue 6 Pages
1077
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Akira Tsujimura, Tadamiki Hihara, Yoshitaka K\={o}i
1962 Volume 17 Issue 6 Pages
1078
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Keigo Nisimura
1962 Volume 17 Issue 6 Pages
1079C
Published: June 05, 1962
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The scales of the ordinates in Figs. 3a, 3b and 3c should be doubled, i.g. “4” in the scales should be read “2”. Line 19 of the right column, page 2100, “94mb” should be read “64mb”.
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Shoji Tauchi
1962 Volume 17 Issue 6 Pages
1079A
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Tsuyoshi Murao
1962 Volume 17 Issue 6 Pages
1079B
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Makoto Kikuchi, Yutaka Abe
1962 Volume 17 Issue 6 Pages
1079D
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The lowest picture in Fig. 3(b) should be rotated 180°.
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